Immediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism

Hydroxylation of arenes via activation of aromatic Csp2–H bond remains a challenge. Here, the authors have managed to get various arenes hydroxylated to corresponding phenols using stoichiometric hydrogen peroxide and a series of robust V–Si–ZSM-22 catalysts synthesized via an ionic liquid involved...

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Autores principales: Yu Zhou, Zhipan Ma, Junjie Tang, Ning Yan, Yonghua Du, Shibo Xi, Kai Wang, Wei Zhang, Haimeng Wen, Jun Wang
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/032d3ab2f1ab440a865646757387ad70
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spelling oai:doaj.org-article:032d3ab2f1ab440a865646757387ad702021-12-02T15:34:26ZImmediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism10.1038/s41467-018-05351-w2041-1723https://doaj.org/article/032d3ab2f1ab440a865646757387ad702018-07-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-05351-whttps://doaj.org/toc/2041-1723Hydroxylation of arenes via activation of aromatic Csp2–H bond remains a challenge. Here, the authors have managed to get various arenes hydroxylated to corresponding phenols using stoichiometric hydrogen peroxide and a series of robust V–Si–ZSM-22 catalysts synthesized via an ionic liquid involved dry-gel-conversion route.Yu ZhouZhipan MaJunjie TangNing YanYonghua DuShibo XiKai WangWei ZhangHaimeng WenJun WangNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-10 (2018)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Yu Zhou
Zhipan Ma
Junjie Tang
Ning Yan
Yonghua Du
Shibo Xi
Kai Wang
Wei Zhang
Haimeng Wen
Jun Wang
Immediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism
description Hydroxylation of arenes via activation of aromatic Csp2–H bond remains a challenge. Here, the authors have managed to get various arenes hydroxylated to corresponding phenols using stoichiometric hydrogen peroxide and a series of robust V–Si–ZSM-22 catalysts synthesized via an ionic liquid involved dry-gel-conversion route.
format article
author Yu Zhou
Zhipan Ma
Junjie Tang
Ning Yan
Yonghua Du
Shibo Xi
Kai Wang
Wei Zhang
Haimeng Wen
Jun Wang
author_facet Yu Zhou
Zhipan Ma
Junjie Tang
Ning Yan
Yonghua Du
Shibo Xi
Kai Wang
Wei Zhang
Haimeng Wen
Jun Wang
author_sort Yu Zhou
title Immediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism
title_short Immediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism
title_full Immediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism
title_fullStr Immediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism
title_full_unstemmed Immediate hydroxylation of arenes to phenols via V-containing all-silica ZSM-22 zeolite triggered non-radical mechanism
title_sort immediate hydroxylation of arenes to phenols via v-containing all-silica zsm-22 zeolite triggered non-radical mechanism
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/032d3ab2f1ab440a865646757387ad70
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