Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
Although it is well known that silica can dissolve in water, the precise mechanism is unclear. Here, the authors employ sum frequency generation spectroscopy to probe the interfacial water structure reporting directly on the underlying dissolution mechanism, which appears to be auto-catalytic.
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Nature Portfolio
2018
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oai:doaj.org-article:039c1ea25d0045709dbaf0c49b2c72e52021-12-02T14:38:49ZEvidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy10.1038/s41467-018-05762-92041-1723https://doaj.org/article/039c1ea25d0045709dbaf0c49b2c72e52018-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-05762-9https://doaj.org/toc/2041-1723Although it is well known that silica can dissolve in water, the precise mechanism is unclear. Here, the authors employ sum frequency generation spectroscopy to probe the interfacial water structure reporting directly on the underlying dissolution mechanism, which appears to be auto-catalytic.Jan SchaeferEllen H. G. BackusMischa BonnNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-6 (2018) |
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Science Q Jan Schaefer Ellen H. G. Backus Mischa Bonn Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy |
description |
Although it is well known that silica can dissolve in water, the precise mechanism is unclear. Here, the authors employ sum frequency generation spectroscopy to probe the interfacial water structure reporting directly on the underlying dissolution mechanism, which appears to be auto-catalytic. |
format |
article |
author |
Jan Schaefer Ellen H. G. Backus Mischa Bonn |
author_facet |
Jan Schaefer Ellen H. G. Backus Mischa Bonn |
author_sort |
Jan Schaefer |
title |
Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy |
title_short |
Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy |
title_full |
Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy |
title_fullStr |
Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy |
title_full_unstemmed |
Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy |
title_sort |
evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy |
publisher |
Nature Portfolio |
publishDate |
2018 |
url |
https://doaj.org/article/039c1ea25d0045709dbaf0c49b2c72e5 |
work_keys_str_mv |
AT janschaefer evidenceforautocatalyticmineraldissolutionfromsurfacespecificvibrationalspectroscopy AT ellenhgbackus evidenceforautocatalyticmineraldissolutionfromsurfacespecificvibrationalspectroscopy AT mischabonn evidenceforautocatalyticmineraldissolutionfromsurfacespecificvibrationalspectroscopy |
_version_ |
1718390811266121728 |