Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy

Although it is well known that silica can dissolve in water, the precise mechanism is unclear. Here, the authors employ sum frequency generation spectroscopy to probe the interfacial water structure reporting directly on the underlying dissolution mechanism, which appears to be auto-catalytic.

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Autores principales: Jan Schaefer, Ellen H. G. Backus, Mischa Bonn
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/039c1ea25d0045709dbaf0c49b2c72e5
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spelling oai:doaj.org-article:039c1ea25d0045709dbaf0c49b2c72e52021-12-02T14:38:49ZEvidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy10.1038/s41467-018-05762-92041-1723https://doaj.org/article/039c1ea25d0045709dbaf0c49b2c72e52018-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-05762-9https://doaj.org/toc/2041-1723Although it is well known that silica can dissolve in water, the precise mechanism is unclear. Here, the authors employ sum frequency generation spectroscopy to probe the interfacial water structure reporting directly on the underlying dissolution mechanism, which appears to be auto-catalytic.Jan SchaeferEllen H. G. BackusMischa BonnNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-6 (2018)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Jan Schaefer
Ellen H. G. Backus
Mischa Bonn
Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
description Although it is well known that silica can dissolve in water, the precise mechanism is unclear. Here, the authors employ sum frequency generation spectroscopy to probe the interfacial water structure reporting directly on the underlying dissolution mechanism, which appears to be auto-catalytic.
format article
author Jan Schaefer
Ellen H. G. Backus
Mischa Bonn
author_facet Jan Schaefer
Ellen H. G. Backus
Mischa Bonn
author_sort Jan Schaefer
title Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
title_short Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
title_full Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
title_fullStr Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
title_full_unstemmed Evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
title_sort evidence for auto-catalytic mineral dissolution from surface-specific vibrational spectroscopy
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/039c1ea25d0045709dbaf0c49b2c72e5
work_keys_str_mv AT janschaefer evidenceforautocatalyticmineraldissolutionfromsurfacespecificvibrationalspectroscopy
AT ellenhgbackus evidenceforautocatalyticmineraldissolutionfromsurfacespecificvibrationalspectroscopy
AT mischabonn evidenceforautocatalyticmineraldissolutionfromsurfacespecificvibrationalspectroscopy
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