Coherent Optical Creation of a Single Molecule

We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large transition dipole moment while reducing photon scattering. Star...

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Auteurs principaux: Yichao Yu, Kenneth Wang, Jonathan D. Hood, Lewis R. B. Picard, Jessie T. Zhang, William B. Cairncross, Jeremy M. Hutson, Rosario Gonzalez-Ferez, Till Rosenband, Kang-Kuen Ni
Format: article
Langue:EN
Publié: American Physical Society 2021
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Accès en ligne:https://doaj.org/article/0616ccbda8ce4e2f8a4ef2a8576d24e5
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Résumé:We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large transition dipole moment while reducing photon scattering. Starting from two atoms in their relative motional ground state, we achieve an optical transfer efficiency of 69%. The molecules have a binding energy of 770.2 MHz at 8.83(2) G. This technique does not rely on Feshbach resonances or narrow excited-state lines and may allow a wide range of molecular species to be assembled atom by atom.