Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites

The rational design of single-atom catalysts is challenging. This work reveals a substrate-strain tuned geometry distortion of CuN2C2 single-atom site, which greatly boosts oxygen reduction activity by facilitating electron transfer to adsorbed O.

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Autores principales:	Guokang Han, Xue Zhang, Wei Liu, Qinghua Zhang, Zhiqiang Wang, Jun Cheng, Tao Yao, Lin Gu, Chunyu Du, Yunzhi Gao, Geping Yin
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2021
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/072f4256cea5454b872c552186885e60
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spelling	oai:doaj.org-article:072f4256cea5454b872c552186885e602021-11-08T11:06:39ZSubstrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites10.1038/s41467-021-26747-12041-1723https://doaj.org/article/072f4256cea5454b872c552186885e602021-11-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-26747-1https://doaj.org/toc/2041-1723The rational design of single-atom catalysts is challenging. This work reveals a substrate-strain tuned geometry distortion of CuN2C2 single-atom site, which greatly boosts oxygen reduction activity by facilitating electron transfer to adsorbed O.Guokang HanXue ZhangWei LiuQinghua ZhangZhiqiang WangJun ChengTao YaoLin GuChunyu DuYunzhi GaoGeping YinNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-9 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Guokang Han Xue Zhang Wei Liu Qinghua Zhang Zhiqiang Wang Jun Cheng Tao Yao Lin Gu Chunyu Du Yunzhi Gao Geping Yin Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites
description	The rational design of single-atom catalysts is challenging. This work reveals a substrate-strain tuned geometry distortion of CuN2C2 single-atom site, which greatly boosts oxygen reduction activity by facilitating electron transfer to adsorbed O.
format	article
author	Guokang Han Xue Zhang Wei Liu Qinghua Zhang Zhiqiang Wang Jun Cheng Tao Yao Lin Gu Chunyu Du Yunzhi Gao Geping Yin
author_facet	Guokang Han Xue Zhang Wei Liu Qinghua Zhang Zhiqiang Wang Jun Cheng Tao Yao Lin Gu Chunyu Du Yunzhi Gao Geping Yin
author_sort	Guokang Han
title	Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites
title_short	Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites
title_full	Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites
title_fullStr	Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites
title_full_unstemmed	Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites
title_sort	substrate strain tunes operando geometric distortion and oxygen reduction activity of cun2c2 single-atom sites
publisher	Nature Portfolio
publishDate	2021
url	https://doaj.org/article/072f4256cea5454b872c552186885e60
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Substrate strain tunes operando geometric distortion and oxygen reduction activity of CuN2C2 single-atom sites

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