Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites

Efficient upgrading of CO to C3 fuel using asymmetric C-C coupling active sites

Catalysts for CO electroreduction have focused on Cu, and their main products have been C2 chemicals. Here authors use the concept of asymmetric active sites to develop a class of doped Cu catalysts for C-C coupling, delivering record selectivity to n-propanol.

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Auteurs principaux: Xue Wang, Ziyun Wang, Tao-Tao Zhuang, Cao-Thang Dinh, Jun Li, Dae-Hyun Nam, Fengwang Li, Chun-Wei Huang, Chih-Shan Tan, Zitao Chen, Miaofang Chi, Christine M. Gabardo, Ali Seifitokaldani, Petar Todorović, Andrew Proppe, Yuanjie Pang, Ahmad R. Kirmani, Yuhang Wang, Alexander H. Ip, Lee J. Richter, Benjamin Scheffel, Aoni Xu, Shen-Chuan Lo, Shana O. Kelley, David Sinton, Edward H. Sargent
Format: article
Langue:EN
Publié: Nature Portfolio 2019
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Science
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Accès en ligne:https://doaj.org/article/07eb2f7d6f2847e28ba2d8860b75cb0b
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Résumé:Catalysts for CO electroreduction have focused on Cu, and their main products have been C2 chemicals. Here authors use the concept of asymmetric active sites to develop a class of doped Cu catalysts for C-C coupling, delivering record selectivity to n-propanol.

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