Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer
Abstract The beneficial use of a hole transport layer (HTL) as a substitution for poly(3,4-ethlyenedioxythiophene): polystyrene sulfonate (PEDOT:PSS) is regarded as one of the most important approaches for improving the stability and efficiency of inverted perovskite solar cells. Here, we demonstrat...
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2018
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oai:doaj.org-article:084069d0e26e4cff8aa66e3c1b4266672021-12-02T15:08:56ZHighly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer10.1038/s41598-018-19612-72045-2322https://doaj.org/article/084069d0e26e4cff8aa66e3c1b4266672018-01-01T00:00:00Zhttps://doi.org/10.1038/s41598-018-19612-7https://doaj.org/toc/2045-2322Abstract The beneficial use of a hole transport layer (HTL) as a substitution for poly(3,4-ethlyenedioxythiophene): polystyrene sulfonate (PEDOT:PSS) is regarded as one of the most important approaches for improving the stability and efficiency of inverted perovskite solar cells. Here, we demonstrate highly efficient and stable inverted perovskite solar cells by applying a GO-doped PEDOT:PSS (PEDOT:GO) film as an HTL. The high performance of this solar cell stems from the excellent optical and electrical properties of the PEDOT:GO film, including a higher electrical conductivity, a higher work function related to the reduced contact barrier between the perovskite layer and the PEDOT:GO layer, enhanced crystallinity of the perovskite crystal, and suppressed leakage current. Moreover, the device with the PEDOT:GO layer showed excellent long-term stability in ambient air conditions. Thus, the enhancement in the efficiency and the excellent stability of inverted perovskite solar cells are promising for the eventual commercialization of perovskite optoelectronic devices.Jae Choul YuJi A HongEui Dae JungDa Bin KimSoo-Min BaekSukbin LeeShinuk ChoSung Soo ParkKyoung Jin ChoiMyoung Hoon SongNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 8, Iss 1, Pp 1-9 (2018) |
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Medicine R Science Q Jae Choul Yu Ji A Hong Eui Dae Jung Da Bin Kim Soo-Min Baek Sukbin Lee Shinuk Cho Sung Soo Park Kyoung Jin Choi Myoung Hoon Song Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer |
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Abstract The beneficial use of a hole transport layer (HTL) as a substitution for poly(3,4-ethlyenedioxythiophene): polystyrene sulfonate (PEDOT:PSS) is regarded as one of the most important approaches for improving the stability and efficiency of inverted perovskite solar cells. Here, we demonstrate highly efficient and stable inverted perovskite solar cells by applying a GO-doped PEDOT:PSS (PEDOT:GO) film as an HTL. The high performance of this solar cell stems from the excellent optical and electrical properties of the PEDOT:GO film, including a higher electrical conductivity, a higher work function related to the reduced contact barrier between the perovskite layer and the PEDOT:GO layer, enhanced crystallinity of the perovskite crystal, and suppressed leakage current. Moreover, the device with the PEDOT:GO layer showed excellent long-term stability in ambient air conditions. Thus, the enhancement in the efficiency and the excellent stability of inverted perovskite solar cells are promising for the eventual commercialization of perovskite optoelectronic devices. |
format |
article |
author |
Jae Choul Yu Ji A Hong Eui Dae Jung Da Bin Kim Soo-Min Baek Sukbin Lee Shinuk Cho Sung Soo Park Kyoung Jin Choi Myoung Hoon Song |
author_facet |
Jae Choul Yu Ji A Hong Eui Dae Jung Da Bin Kim Soo-Min Baek Sukbin Lee Shinuk Cho Sung Soo Park Kyoung Jin Choi Myoung Hoon Song |
author_sort |
Jae Choul Yu |
title |
Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer |
title_short |
Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer |
title_full |
Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer |
title_fullStr |
Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer |
title_full_unstemmed |
Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer |
title_sort |
highly efficient and stable inverted perovskite solar cell employing pedot:go composite layer as a hole transport layer |
publisher |
Nature Portfolio |
publishDate |
2018 |
url |
https://doaj.org/article/084069d0e26e4cff8aa66e3c1b426667 |
work_keys_str_mv |
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