Active site localization of methane oxidation on Pt nanocrystals

The structural changes at low-coordination sites of nanocatalysts such as edges, remain poorly understood. Here, the authors report observations of high-lattice distortion at edges of Pt nanocrystals during heterogeneous catalytic methane oxidation by using in situ 3D Bragg coherent X-ray diffractio...

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Autores principales: Dongjin Kim, Myungwoo Chung, Jerome Carnis, Sungwon Kim, Kyuseok Yun, Jinback Kang, Wonsuk Cha, Mathew J. Cherukara, Evan Maxey, Ross Harder, Kiran Sasikumar, Subramanian K. R. S. Sankaranarayanan, Alexey Zozulya, Michael Sprung, Dohhyung Riu, Hyunjung Kim
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/0b9b6c370e87408ea14d796282f7a495
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spelling oai:doaj.org-article:0b9b6c370e87408ea14d796282f7a4952021-12-02T14:39:04ZActive site localization of methane oxidation on Pt nanocrystals10.1038/s41467-018-05464-22041-1723https://doaj.org/article/0b9b6c370e87408ea14d796282f7a4952018-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-05464-2https://doaj.org/toc/2041-1723The structural changes at low-coordination sites of nanocatalysts such as edges, remain poorly understood. Here, the authors report observations of high-lattice distortion at edges of Pt nanocrystals during heterogeneous catalytic methane oxidation by using in situ 3D Bragg coherent X-ray diffraction imaging.Dongjin KimMyungwoo ChungJerome CarnisSungwon KimKyuseok YunJinback KangWonsuk ChaMathew J. CherukaraEvan MaxeyRoss HarderKiran SasikumarSubramanian K. R. S. SankaranarayananAlexey ZozulyaMichael SprungDohhyung RiuHyunjung KimNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-7 (2018)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Dongjin Kim
Myungwoo Chung
Jerome Carnis
Sungwon Kim
Kyuseok Yun
Jinback Kang
Wonsuk Cha
Mathew J. Cherukara
Evan Maxey
Ross Harder
Kiran Sasikumar
Subramanian K. R. S. Sankaranarayanan
Alexey Zozulya
Michael Sprung
Dohhyung Riu
Hyunjung Kim
Active site localization of methane oxidation on Pt nanocrystals
description The structural changes at low-coordination sites of nanocatalysts such as edges, remain poorly understood. Here, the authors report observations of high-lattice distortion at edges of Pt nanocrystals during heterogeneous catalytic methane oxidation by using in situ 3D Bragg coherent X-ray diffraction imaging.
format article
author Dongjin Kim
Myungwoo Chung
Jerome Carnis
Sungwon Kim
Kyuseok Yun
Jinback Kang
Wonsuk Cha
Mathew J. Cherukara
Evan Maxey
Ross Harder
Kiran Sasikumar
Subramanian K. R. S. Sankaranarayanan
Alexey Zozulya
Michael Sprung
Dohhyung Riu
Hyunjung Kim
author_facet Dongjin Kim
Myungwoo Chung
Jerome Carnis
Sungwon Kim
Kyuseok Yun
Jinback Kang
Wonsuk Cha
Mathew J. Cherukara
Evan Maxey
Ross Harder
Kiran Sasikumar
Subramanian K. R. S. Sankaranarayanan
Alexey Zozulya
Michael Sprung
Dohhyung Riu
Hyunjung Kim
author_sort Dongjin Kim
title Active site localization of methane oxidation on Pt nanocrystals
title_short Active site localization of methane oxidation on Pt nanocrystals
title_full Active site localization of methane oxidation on Pt nanocrystals
title_fullStr Active site localization of methane oxidation on Pt nanocrystals
title_full_unstemmed Active site localization of methane oxidation on Pt nanocrystals
title_sort active site localization of methane oxidation on pt nanocrystals
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/0b9b6c370e87408ea14d796282f7a495
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