Coherent vibrational dynamics reveals lattice anharmonicity in organic–inorganic halide perovskite nanocrystals
Using a combination of femtosecond pump-probe spectroscopy and first-principles calculations, Debnath et al. elucidated the halide-dependence of the excited state vibrational coherences in hybrid organic-inorganic perovskite nanocrystals. The study revealed an intrinsic anharmonicity of lead-halide...
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| Autores principales: | , , , , , , , |
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| Formato: | article |
| Lenguaje: | EN |
| Publicado: |
Nature Portfolio
2021
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| Materias: | |
| Acceso en línea: | https://doaj.org/article/0d36d7aa0b3c4467b1eb1d8fc193c1da |
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| Sumario: | Using a combination of femtosecond pump-probe spectroscopy and first-principles calculations, Debnath et al. elucidated the halide-dependence of the excited state vibrational coherences in hybrid organic-inorganic perovskite nanocrystals. The study revealed an intrinsic anharmonicity of lead-halide framework, which correlates with perovskite stability and is influenced by the interaction between the framework and the organic molecules. |
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