The dark exciton ground state promotes photon-pair emission in individual perovskite nanocrystals

The optical and electronic properties of cesium lead halide perovskite nanocrystals are dictated by the band-edge exciton, whose physics is not elucidated. Here, the authors unveil its fine structure and demonstrate that the ground dark singlet state promotes the creation of biexcitons at low temper...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autores principales: Philippe Tamarat, Lei Hou, Jean-Baptiste Trebbia, Abhishek Swarnkar, Louis Biadala, Yann Louyer, Maryna I. Bodnarchuk, Maksym V. Kovalenko, Jacky Even, Brahim Lounis
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2020
Materias:
Q
Acceso en línea:https://doaj.org/article/0e88587303554578988db2993be04e79
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
Descripción
Sumario:The optical and electronic properties of cesium lead halide perovskite nanocrystals are dictated by the band-edge exciton, whose physics is not elucidated. Here, the authors unveil its fine structure and demonstrate that the ground dark singlet state promotes the creation of biexcitons at low temperatures and thus correlated photon pairs.