Alcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors

Abstract Chemical sensors detect a variety of chemicals across numerous fields, such as automobile, aerospace, safety, indoor air quality, environmental control, food, industrial production and medicine. We successfully assemble an alcohol-sensing device comprising a thin-film sensor made of graphen...

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Autores principales: Xuezhu Xu, Jian Zhou, Yangyang Xin, Gilles Lubineau, Qian Ma, Long Jiang
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Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/0f48167d8bc74d33b424c4f939f37fc3
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spelling oai:doaj.org-article:0f48167d8bc74d33b424c4f939f37fc32021-12-02T12:30:36ZAlcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors10.1038/s41598-017-04636-22045-2322https://doaj.org/article/0f48167d8bc74d33b424c4f939f37fc32017-06-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-04636-2https://doaj.org/toc/2045-2322Abstract Chemical sensors detect a variety of chemicals across numerous fields, such as automobile, aerospace, safety, indoor air quality, environmental control, food, industrial production and medicine. We successfully assemble an alcohol-sensing device comprising a thin-film sensor made of graphene nanosheets (GNs) and bacterial cellulose nanofibers (BCNs). We show that the GN/BCN sensor has a high selectivity to ethanol by distinguishing liquid–phase or vapor–phase ethanol (C2H6O) from water (H2O) intelligently with accurate transformation into electrical signals in devices. The BCN component of the film amplifies the ethanol sensitivity of the film, whereby the GN/BCN sensor has 12400% sensitivity for vapor-phase ethanol compared to the pure GN sensor, which has only 21% sensitivity. Finally, GN/BCN sensors demonstrate fast response/recovery times and a wide range of alcohol detection (10–100%). The superior sensing ability of GN/BCN compared to GNs alone is due to the improved wettability of BCNs and the ionization of liquids. We prove a facile, green, low-cost route for the assembly of ethanol-sensing devices with potential for vast application.Xuezhu XuJian ZhouYangyang XinGilles LubineauQian MaLong JiangNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-10 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Xuezhu Xu
Jian Zhou
Yangyang Xin
Gilles Lubineau
Qian Ma
Long Jiang
Alcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors
description Abstract Chemical sensors detect a variety of chemicals across numerous fields, such as automobile, aerospace, safety, indoor air quality, environmental control, food, industrial production and medicine. We successfully assemble an alcohol-sensing device comprising a thin-film sensor made of graphene nanosheets (GNs) and bacterial cellulose nanofibers (BCNs). We show that the GN/BCN sensor has a high selectivity to ethanol by distinguishing liquid–phase or vapor–phase ethanol (C2H6O) from water (H2O) intelligently with accurate transformation into electrical signals in devices. The BCN component of the film amplifies the ethanol sensitivity of the film, whereby the GN/BCN sensor has 12400% sensitivity for vapor-phase ethanol compared to the pure GN sensor, which has only 21% sensitivity. Finally, GN/BCN sensors demonstrate fast response/recovery times and a wide range of alcohol detection (10–100%). The superior sensing ability of GN/BCN compared to GNs alone is due to the improved wettability of BCNs and the ionization of liquids. We prove a facile, green, low-cost route for the assembly of ethanol-sensing devices with potential for vast application.
format article
author Xuezhu Xu
Jian Zhou
Yangyang Xin
Gilles Lubineau
Qian Ma
Long Jiang
author_facet Xuezhu Xu
Jian Zhou
Yangyang Xin
Gilles Lubineau
Qian Ma
Long Jiang
author_sort Xuezhu Xu
title Alcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors
title_short Alcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors
title_full Alcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors
title_fullStr Alcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors
title_full_unstemmed Alcohol Recognition by Flexible, Transparent and Highly Sensitive Graphene-Based Thin-Film Sensors
title_sort alcohol recognition by flexible, transparent and highly sensitive graphene-based thin-film sensors
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/0f48167d8bc74d33b424c4f939f37fc3
work_keys_str_mv AT xuezhuxu alcoholrecognitionbyflexibletransparentandhighlysensitivegraphenebasedthinfilmsensors
AT jianzhou alcoholrecognitionbyflexibletransparentandhighlysensitivegraphenebasedthinfilmsensors
AT yangyangxin alcoholrecognitionbyflexibletransparentandhighlysensitivegraphenebasedthinfilmsensors
AT gilleslubineau alcoholrecognitionbyflexibletransparentandhighlysensitivegraphenebasedthinfilmsensors
AT qianma alcoholrecognitionbyflexibletransparentandhighlysensitivegraphenebasedthinfilmsensors
AT longjiang alcoholrecognitionbyflexibletransparentandhighlysensitivegraphenebasedthinfilmsensors
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