Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis

CO2-to-ethylene conversion using renewable electricity provides a sustainable route to produce valuable chemicals. Here, the authors report high ethylene activity of 215 mA cm−2 and selectivity of 65% made possible by silica clusters in copper.

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Autores principales: Jun Li, Adnan Ozden, Mingyu Wan, Yongfeng Hu, Fengwang Li, Yuhang Wang, Reza R. Zamani, Dan Ren, Ziyun Wang, Yi Xu, Dae-Hyun Nam, Joshua Wicks, Bin Chen, Xue Wang, Mingchuan Luo, Michael Graetzel, Fanglin Che, Edward H. Sargent, David Sinton
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/126836d713604c1aa03a09a4261d0cdd
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spelling oai:doaj.org-article:126836d713604c1aa03a09a4261d0cdd2021-12-02T16:50:30ZSilica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis10.1038/s41467-021-23023-02041-1723https://doaj.org/article/126836d713604c1aa03a09a4261d0cdd2021-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-23023-0https://doaj.org/toc/2041-1723CO2-to-ethylene conversion using renewable electricity provides a sustainable route to produce valuable chemicals. Here, the authors report high ethylene activity of 215 mA cm−2 and selectivity of 65% made possible by silica clusters in copper.Jun LiAdnan OzdenMingyu WanYongfeng HuFengwang LiYuhang WangReza R. ZamaniDan RenZiyun WangYi XuDae-Hyun NamJoshua WicksBin ChenXue WangMingchuan LuoMichael GraetzelFanglin CheEdward H. SargentDavid SintonNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-10 (2021)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Jun Li
Adnan Ozden
Mingyu Wan
Yongfeng Hu
Fengwang Li
Yuhang Wang
Reza R. Zamani
Dan Ren
Ziyun Wang
Yi Xu
Dae-Hyun Nam
Joshua Wicks
Bin Chen
Xue Wang
Mingchuan Luo
Michael Graetzel
Fanglin Che
Edward H. Sargent
David Sinton
Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis
description CO2-to-ethylene conversion using renewable electricity provides a sustainable route to produce valuable chemicals. Here, the authors report high ethylene activity of 215 mA cm−2 and selectivity of 65% made possible by silica clusters in copper.
format article
author Jun Li
Adnan Ozden
Mingyu Wan
Yongfeng Hu
Fengwang Li
Yuhang Wang
Reza R. Zamani
Dan Ren
Ziyun Wang
Yi Xu
Dae-Hyun Nam
Joshua Wicks
Bin Chen
Xue Wang
Mingchuan Luo
Michael Graetzel
Fanglin Che
Edward H. Sargent
David Sinton
author_facet Jun Li
Adnan Ozden
Mingyu Wan
Yongfeng Hu
Fengwang Li
Yuhang Wang
Reza R. Zamani
Dan Ren
Ziyun Wang
Yi Xu
Dae-Hyun Nam
Joshua Wicks
Bin Chen
Xue Wang
Mingchuan Luo
Michael Graetzel
Fanglin Che
Edward H. Sargent
David Sinton
author_sort Jun Li
title Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis
title_short Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis
title_full Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis
title_fullStr Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis
title_full_unstemmed Silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis
title_sort silica-copper catalyst interfaces enable carbon-carbon coupling towards ethylene electrosynthesis
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/126836d713604c1aa03a09a4261d0cdd
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AT yongfenghu silicacoppercatalystinterfacesenablecarboncarboncouplingtowardsethyleneelectrosynthesis
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