Modeling and mapping of atmospheric mercury deposition in adirondack park, new york.
The Adirondacks of New York State, USA is a region that is sensitive to atmospheric mercury (Hg) deposition. In this study, we estimated atmospheric Hg deposition to the Adirondacks using a new scheme that combined numerical modeling and limited experimental data. The majority of the land cover in t...
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2013
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oai:doaj.org-article:159057bce1484e9da016d86b0bbc7de72021-11-18T07:52:09ZModeling and mapping of atmospheric mercury deposition in adirondack park, new york.1932-620310.1371/journal.pone.0059322https://doaj.org/article/159057bce1484e9da016d86b0bbc7de72013-01-01T00:00:00Zhttps://www.ncbi.nlm.nih.gov/pmc/articles/pmid/23536871/pdf/?tool=EBIhttps://doaj.org/toc/1932-6203The Adirondacks of New York State, USA is a region that is sensitive to atmospheric mercury (Hg) deposition. In this study, we estimated atmospheric Hg deposition to the Adirondacks using a new scheme that combined numerical modeling and limited experimental data. The majority of the land cover in the Adirondacks is forested with 47% of the total area deciduous, 20% coniferous and 10% mixed. We used litterfall plus throughfall deposition as the total atmospheric Hg deposition to coniferous and deciduous forests during the leaf-on period, and wet Hg deposition plus modeled atmospheric dry Hg deposition as the total Hg deposition to the deciduous forest during the leaf-off period and for the non-forested areas year-around. To estimate atmospheric dry Hg deposition we used the Big Leaf model. The average atmospheric Hg deposition to the Adirondacks was estimated as 17.4 [Formula: see text]g m[Formula: see text] yr[Formula: see text] with a range of -3.7-46.0 [Formula: see text]g m[Formula: see text] yr[Formula: see text]. Atmospheric Hg dry deposition (370 kg yr[Formula: see text]) was found to be more important than wet deposition (210 kg yr[Formula: see text]) to the entire Adirondacks (2.4 million ha). The spatial pattern showed a large variation in atmospheric Hg deposition with scattered areas in the eastern Adirondacks having total Hg deposition greater than 30 μg m(-2) yr(-1), while the southwestern and the northern areas received Hg deposition ranging from 25-30 μg m(-2) yr(-1).Xue YuCharles T DriscollJiaoyan HuangThomas M HolsenBradley D BlackwellPublic Library of Science (PLoS)articleMedicineRScienceQENPLoS ONE, Vol 8, Iss 3, p e59322 (2013) |
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Medicine R Science Q Xue Yu Charles T Driscoll Jiaoyan Huang Thomas M Holsen Bradley D Blackwell Modeling and mapping of atmospheric mercury deposition in adirondack park, new york. |
description |
The Adirondacks of New York State, USA is a region that is sensitive to atmospheric mercury (Hg) deposition. In this study, we estimated atmospheric Hg deposition to the Adirondacks using a new scheme that combined numerical modeling and limited experimental data. The majority of the land cover in the Adirondacks is forested with 47% of the total area deciduous, 20% coniferous and 10% mixed. We used litterfall plus throughfall deposition as the total atmospheric Hg deposition to coniferous and deciduous forests during the leaf-on period, and wet Hg deposition plus modeled atmospheric dry Hg deposition as the total Hg deposition to the deciduous forest during the leaf-off period and for the non-forested areas year-around. To estimate atmospheric dry Hg deposition we used the Big Leaf model. The average atmospheric Hg deposition to the Adirondacks was estimated as 17.4 [Formula: see text]g m[Formula: see text] yr[Formula: see text] with a range of -3.7-46.0 [Formula: see text]g m[Formula: see text] yr[Formula: see text]. Atmospheric Hg dry deposition (370 kg yr[Formula: see text]) was found to be more important than wet deposition (210 kg yr[Formula: see text]) to the entire Adirondacks (2.4 million ha). The spatial pattern showed a large variation in atmospheric Hg deposition with scattered areas in the eastern Adirondacks having total Hg deposition greater than 30 μg m(-2) yr(-1), while the southwestern and the northern areas received Hg deposition ranging from 25-30 μg m(-2) yr(-1). |
format |
article |
author |
Xue Yu Charles T Driscoll Jiaoyan Huang Thomas M Holsen Bradley D Blackwell |
author_facet |
Xue Yu Charles T Driscoll Jiaoyan Huang Thomas M Holsen Bradley D Blackwell |
author_sort |
Xue Yu |
title |
Modeling and mapping of atmospheric mercury deposition in adirondack park, new york. |
title_short |
Modeling and mapping of atmospheric mercury deposition in adirondack park, new york. |
title_full |
Modeling and mapping of atmospheric mercury deposition in adirondack park, new york. |
title_fullStr |
Modeling and mapping of atmospheric mercury deposition in adirondack park, new york. |
title_full_unstemmed |
Modeling and mapping of atmospheric mercury deposition in adirondack park, new york. |
title_sort |
modeling and mapping of atmospheric mercury deposition in adirondack park, new york. |
publisher |
Public Library of Science (PLoS) |
publishDate |
2013 |
url |
https://doaj.org/article/159057bce1484e9da016d86b0bbc7de7 |
work_keys_str_mv |
AT xueyu modelingandmappingofatmosphericmercurydepositioninadirondackparknewyork AT charlestdriscoll modelingandmappingofatmosphericmercurydepositioninadirondackparknewyork AT jiaoyanhuang modelingandmappingofatmosphericmercurydepositioninadirondackparknewyork AT thomasmholsen modelingandmappingofatmosphericmercurydepositioninadirondackparknewyork AT bradleydblackwell modelingandmappingofatmosphericmercurydepositioninadirondackparknewyork |
_version_ |
1718422836239925248 |