Dynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction
Revealing the structure and dynamics of active sites is essential to understand catalytic mechanisms. Here the authors demonstrate the dynamic nature of perimeter Pt0−O vacancy−Ce3+ sites in Pt/CeO2 and the key effects of their dynamics on the mechanism of the water gas shift reaction.
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Nature Portfolio
2021
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oai:doaj.org-article:162febbfa3814d3abbe2585eb3a7b0852021-12-02T13:30:07ZDynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction10.1038/s41467-021-21132-42041-1723https://doaj.org/article/162febbfa3814d3abbe2585eb3a7b0852021-02-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-21132-4https://doaj.org/toc/2041-1723Revealing the structure and dynamics of active sites is essential to understand catalytic mechanisms. Here the authors demonstrate the dynamic nature of perimeter Pt0−O vacancy−Ce3+ sites in Pt/CeO2 and the key effects of their dynamics on the mechanism of the water gas shift reaction.Yuanyuan LiMatthew KottwitzJoshua L. VincentMichael J. EnrightZongyuan LiuLihua ZhangJiahao HuangSanjaya D. SenanayakeWei-Chang D. YangPeter A. CrozierRalph G. NuzzoAnatoly I. FrenkelNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-9 (2021) |
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Science Q |
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Science Q Yuanyuan Li Matthew Kottwitz Joshua L. Vincent Michael J. Enright Zongyuan Liu Lihua Zhang Jiahao Huang Sanjaya D. Senanayake Wei-Chang D. Yang Peter A. Crozier Ralph G. Nuzzo Anatoly I. Frenkel Dynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction |
description |
Revealing the structure and dynamics of active sites is essential to understand catalytic mechanisms. Here the authors demonstrate the dynamic nature of perimeter Pt0−O vacancy−Ce3+ sites in Pt/CeO2 and the key effects of their dynamics on the mechanism of the water gas shift reaction. |
format |
article |
author |
Yuanyuan Li Matthew Kottwitz Joshua L. Vincent Michael J. Enright Zongyuan Liu Lihua Zhang Jiahao Huang Sanjaya D. Senanayake Wei-Chang D. Yang Peter A. Crozier Ralph G. Nuzzo Anatoly I. Frenkel |
author_facet |
Yuanyuan Li Matthew Kottwitz Joshua L. Vincent Michael J. Enright Zongyuan Liu Lihua Zhang Jiahao Huang Sanjaya D. Senanayake Wei-Chang D. Yang Peter A. Crozier Ralph G. Nuzzo Anatoly I. Frenkel |
author_sort |
Yuanyuan Li |
title |
Dynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction |
title_short |
Dynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction |
title_full |
Dynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction |
title_fullStr |
Dynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction |
title_full_unstemmed |
Dynamic structure of active sites in ceria-supported Pt catalysts for the water gas shift reaction |
title_sort |
dynamic structure of active sites in ceria-supported pt catalysts for the water gas shift reaction |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/162febbfa3814d3abbe2585eb3a7b085 |
work_keys_str_mv |
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1718392957901471744 |