Graphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review

Fenton-like reactions represent an effective strategy to generate strongly oxidative species for the elimination of refractory organic pollutants in water. In the past decades, many research efforts have been made to the development of heterogeneous catalysts in Fenton-like reaction, in order to add...

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Autores principales: Lingling Wang, Yuwei Zhang, Jieshu Qian
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Lenguaje:EN
Publicado: Elsevier 2021
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Acceso en línea:https://doaj.org/article/16ea261443f04d2ea206f114b990ac4f
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spelling oai:doaj.org-article:16ea261443f04d2ea206f114b990ac4f2021-11-18T04:53:05ZGraphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review2666-821110.1016/j.ceja.2021.100171https://doaj.org/article/16ea261443f04d2ea206f114b990ac4f2021-11-01T00:00:00Zhttp://www.sciencedirect.com/science/article/pii/S2666821121000879https://doaj.org/toc/2666-8211Fenton-like reactions represent an effective strategy to generate strongly oxidative species for the elimination of refractory organic pollutants in water. In the past decades, many research efforts have been made to the development of heterogeneous catalysts in Fenton-like reaction, in order to address the issues in homogeneous Fenton system, e.g., narrow pH suitability, slow reduction of Fe3+ to Fe2+, and production of iron sludge. Graphene aerogel (GA), with unique π-π conjugated structure and properties, has been widely used in many applications, including as substrate for the preparation of composite catalysts used in various reactions. In this review, we summarize recent studies using GA as substrate for the preparation of heterogeneous catalysts in Fenton-like reactions. We first describe briefly the preparation of GA and GA-based composites. We then separate the examples of GA-based catalysts in three chapters, i.e., in conventional Fenton, photo-Fenton, and electro-Fenton systems. The mechanisms for the enhancement of catalytic reactivity in these Fenton-like systems due to the use of GA are also discussed. In the end, future studies are envisioned.Lingling WangYuwei ZhangJieshu QianElsevierarticleGraphene aerogelFenton-like reactionHeterogeneous catalystWater treatmentChemical engineeringTP155-156ENChemical Engineering Journal Advances, Vol 8, Iss , Pp 100171- (2021)
institution DOAJ
collection DOAJ
language EN
topic Graphene aerogel
Fenton-like reaction
Heterogeneous catalyst
Water treatment
Chemical engineering
TP155-156
spellingShingle Graphene aerogel
Fenton-like reaction
Heterogeneous catalyst
Water treatment
Chemical engineering
TP155-156
Lingling Wang
Yuwei Zhang
Jieshu Qian
Graphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review
description Fenton-like reactions represent an effective strategy to generate strongly oxidative species for the elimination of refractory organic pollutants in water. In the past decades, many research efforts have been made to the development of heterogeneous catalysts in Fenton-like reaction, in order to address the issues in homogeneous Fenton system, e.g., narrow pH suitability, slow reduction of Fe3+ to Fe2+, and production of iron sludge. Graphene aerogel (GA), with unique π-π conjugated structure and properties, has been widely used in many applications, including as substrate for the preparation of composite catalysts used in various reactions. In this review, we summarize recent studies using GA as substrate for the preparation of heterogeneous catalysts in Fenton-like reactions. We first describe briefly the preparation of GA and GA-based composites. We then separate the examples of GA-based catalysts in three chapters, i.e., in conventional Fenton, photo-Fenton, and electro-Fenton systems. The mechanisms for the enhancement of catalytic reactivity in these Fenton-like systems due to the use of GA are also discussed. In the end, future studies are envisioned.
format article
author Lingling Wang
Yuwei Zhang
Jieshu Qian
author_facet Lingling Wang
Yuwei Zhang
Jieshu Qian
author_sort Lingling Wang
title Graphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review
title_short Graphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review
title_full Graphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review
title_fullStr Graphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review
title_full_unstemmed Graphene aerogel-based catalysts in Fenton-like reactions for water decontamination: a short review
title_sort graphene aerogel-based catalysts in fenton-like reactions for water decontamination: a short review
publisher Elsevier
publishDate 2021
url https://doaj.org/article/16ea261443f04d2ea206f114b990ac4f
work_keys_str_mv AT linglingwang grapheneaerogelbasedcatalystsinfentonlikereactionsforwaterdecontaminationashortreview
AT yuweizhang grapheneaerogelbasedcatalystsinfentonlikereactionsforwaterdecontaminationashortreview
AT jieshuqian grapheneaerogelbasedcatalystsinfentonlikereactionsforwaterdecontaminationashortreview
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