The solution plasma process for heteroatom-carbon nanosheets: the role of precursors

Abstract The solution plasma process (SPP), known as non-equilibrium cold plasma at atmospheric pressure and room temperature, was used to investigate the synthesis of nitrogen-carbon nasnosheets (NCNs). To verify the effect of elementary composition and structure of N-methyl-2-pyrrolidone (NMP), va...

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Autores principales: Koangyong Hyun, Nagahiro Saito
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Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/1837b6edfeda4f309fef2c872429dffb
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spelling oai:doaj.org-article:1837b6edfeda4f309fef2c872429dffb2021-12-02T12:30:24ZThe solution plasma process for heteroatom-carbon nanosheets: the role of precursors10.1038/s41598-017-04190-x2045-2322https://doaj.org/article/1837b6edfeda4f309fef2c872429dffb2017-06-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-04190-xhttps://doaj.org/toc/2045-2322Abstract The solution plasma process (SPP), known as non-equilibrium cold plasma at atmospheric pressure and room temperature, was used to investigate the synthesis of nitrogen-carbon nasnosheets (NCNs). To verify the effect of elementary composition and structure of N-methyl-2-pyrrolidone (NMP), various precursors were used in the SPP to synthesize NCNs via the bottom-up synthesis method for the first time. The NCNs were analyzed by transmission electron microscopy, Raman spectroscopy, and X-ray photoelectron spectroscopy. Among the various precursors, SPP of 2-pyrrolidone was demonstrated to facilitate the formation of highly ordered NCNs. On the other hand, the SPP with cyclopentanone, cyclohexanone and pyrrole did not lead to the formation of carbon nanosheets. The results of this study would uncover new parameter fields for the growth of heteroatom-carbon nanosheets using this synthesis system. In addition, the study is expected to contribute toward research in improving the large-area growth and quality of two-dimensional nanostructures, such as heteroatom-carbon nanosheets or graphene, for various applications in other synthesis methods.Koangyong HyunNagahiro SaitoNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Koangyong Hyun
Nagahiro Saito
The solution plasma process for heteroatom-carbon nanosheets: the role of precursors
description Abstract The solution plasma process (SPP), known as non-equilibrium cold plasma at atmospheric pressure and room temperature, was used to investigate the synthesis of nitrogen-carbon nasnosheets (NCNs). To verify the effect of elementary composition and structure of N-methyl-2-pyrrolidone (NMP), various precursors were used in the SPP to synthesize NCNs via the bottom-up synthesis method for the first time. The NCNs were analyzed by transmission electron microscopy, Raman spectroscopy, and X-ray photoelectron spectroscopy. Among the various precursors, SPP of 2-pyrrolidone was demonstrated to facilitate the formation of highly ordered NCNs. On the other hand, the SPP with cyclopentanone, cyclohexanone and pyrrole did not lead to the formation of carbon nanosheets. The results of this study would uncover new parameter fields for the growth of heteroatom-carbon nanosheets using this synthesis system. In addition, the study is expected to contribute toward research in improving the large-area growth and quality of two-dimensional nanostructures, such as heteroatom-carbon nanosheets or graphene, for various applications in other synthesis methods.
format article
author Koangyong Hyun
Nagahiro Saito
author_facet Koangyong Hyun
Nagahiro Saito
author_sort Koangyong Hyun
title The solution plasma process for heteroatom-carbon nanosheets: the role of precursors
title_short The solution plasma process for heteroatom-carbon nanosheets: the role of precursors
title_full The solution plasma process for heteroatom-carbon nanosheets: the role of precursors
title_fullStr The solution plasma process for heteroatom-carbon nanosheets: the role of precursors
title_full_unstemmed The solution plasma process for heteroatom-carbon nanosheets: the role of precursors
title_sort solution plasma process for heteroatom-carbon nanosheets: the role of precursors
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/1837b6edfeda4f309fef2c872429dffb
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