On the low reinforcing efficiency of carbon nanotubes in high performance polymer fibres

Driven by the exceptionally high mechanical properties of carbon nanotubes (CNTs), over the years an extensive research effort has been devoted to the reinforcement of high-performance polymer fibres with CNTs. However, to date, improvements in the strength of these fibres have been rather modest ev...

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Autores principales: Stergios Goutianos, Ton Peijs
Formato: article
Lenguaje:EN
Publicado: Taylor & Francis Group 2021
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Acceso en línea:https://doaj.org/article/1b9c3f213ff94b0b97f155d1d053dd91
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Sumario:Driven by the exceptionally high mechanical properties of carbon nanotubes (CNTs), over the years an extensive research effort has been devoted to the reinforcement of high-performance polymer fibres with CNTs. However, to date, improvements in the strength of these fibres have been rather modest even for relatively high CNT contents. After a brief review of CNT reinforced polymer fibres, here, analytical and numerical models will be used to show that these experimental findings are to be expected based on the intrinsic mechanical properties of these polymer fibres and CNTs, their aspect ratio and interfacial characteristics. Results show that for realistic CNT contents and aspect ratios, the extraordinary strength of CNTs cannot be fully exploited in high-performance polymer fibres like Dyneema® or Kevlar®, even if these CNTs are perfectly aligned and homogeneously dispersed, due to the low intrinsic shear strength of these highly anisotropic fibres.