Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities
Abstract We investigate the generation of ultraviolet (UV) second-harmonic radiation at the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By adhering to another UV non-transparent crystal with...
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2018
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oai:doaj.org-article:1d963f45e8774be8bac34d0e3d7bdc6d2021-12-02T15:05:30ZEnhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities10.1038/s41598-018-25041-32045-2322https://doaj.org/article/1d963f45e8774be8bac34d0e3d7bdc6d2018-04-01T00:00:00Zhttps://doi.org/10.1038/s41598-018-25041-3https://doaj.org/toc/2045-2322Abstract We investigate the generation of ultraviolet (UV) second-harmonic radiation at the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By adhering to another UV non-transparent crystal with a larger second-order nonlinear coefficient χ (2), a nonlinear interface with large disparity in χ (2) is formed and the enhancement of UV second-harmonic radiation is observed experimentally. The intensity of enhanced second harmonic wave generated at the nonlinear interface is up to 11.6 times that at the crystal boundary. As a tunable phase-matching method, it may suggest potential applications in the UV, and even vacuum-UV region.Xiaohui ZhaoYuanlin ZhengNing AnHuaijin RenXuewei DengXianfeng ChenNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 8, Iss 1, Pp 1-6 (2018) |
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Medicine R Science Q Xiaohui Zhao Yuanlin Zheng Ning An Huaijin Ren Xuewei Deng Xianfeng Chen Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities |
description |
Abstract We investigate the generation of ultraviolet (UV) second-harmonic radiation at the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By adhering to another UV non-transparent crystal with a larger second-order nonlinear coefficient χ (2), a nonlinear interface with large disparity in χ (2) is formed and the enhancement of UV second-harmonic radiation is observed experimentally. The intensity of enhanced second harmonic wave generated at the nonlinear interface is up to 11.6 times that at the crystal boundary. As a tunable phase-matching method, it may suggest potential applications in the UV, and even vacuum-UV region. |
format |
article |
author |
Xiaohui Zhao Yuanlin Zheng Ning An Huaijin Ren Xuewei Deng Xianfeng Chen |
author_facet |
Xiaohui Zhao Yuanlin Zheng Ning An Huaijin Ren Xuewei Deng Xianfeng Chen |
author_sort |
Xiaohui Zhao |
title |
Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities |
title_short |
Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities |
title_full |
Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities |
title_fullStr |
Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities |
title_full_unstemmed |
Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities |
title_sort |
enhancement of uv second-harmonic radiation at nonlinear interfaces with discontinuous second-order susceptibilities |
publisher |
Nature Portfolio |
publishDate |
2018 |
url |
https://doaj.org/article/1d963f45e8774be8bac34d0e3d7bdc6d |
work_keys_str_mv |
AT xiaohuizhao enhancementofuvsecondharmonicradiationatnonlinearinterfaceswithdiscontinuoussecondordersusceptibilities AT yuanlinzheng enhancementofuvsecondharmonicradiationatnonlinearinterfaceswithdiscontinuoussecondordersusceptibilities AT ningan enhancementofuvsecondharmonicradiationatnonlinearinterfaceswithdiscontinuoussecondordersusceptibilities AT huaijinren enhancementofuvsecondharmonicradiationatnonlinearinterfaceswithdiscontinuoussecondordersusceptibilities AT xueweideng enhancementofuvsecondharmonicradiationatnonlinearinterfaceswithdiscontinuoussecondordersusceptibilities AT xianfengchen enhancementofuvsecondharmonicradiationatnonlinearinterfaceswithdiscontinuoussecondordersusceptibilities |
_version_ |
1718388816252764160 |