Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling

<p>Due to its dryness, the subtropical free troposphere plays a critical role in the radiative balance of the Earth's climate system. But the complex interactions of the dynamical and physical processes controlling the variability in the moisture budget of this sensitive region of the sub...

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Autores principales: F. Dahinden, F. Aemisegger, H. Wernli, M. Schneider, C. J. Diekmann, B. Ertl, P. Knippertz, M. Werner, S. Pfahl
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Lenguaje:EN
Publicado: Copernicus Publications 2021
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id oai:doaj.org-article:20c76147d9644ddfaf7ef671937076d9
record_format dspace
institution DOAJ
collection DOAJ
language EN
topic Physics
QC1-999
Chemistry
QD1-999
spellingShingle Physics
QC1-999
Chemistry
QD1-999
F. Dahinden
F. Aemisegger
H. Wernli
M. Schneider
C. J. Diekmann
B. Ertl
P. Knippertz
M. Werner
S. Pfahl
Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling
description <p>Due to its dryness, the subtropical free troposphere plays a critical role in the radiative balance of the Earth's climate system. But the complex interactions of the dynamical and physical processes controlling the variability in the moisture budget of this sensitive region of the subtropical atmosphere are still not fully understood. Stable water isotopes can provide important information about several of the latter processes, namely subsidence drying, turbulent mixing, and dry and moist convective moistening. In this study, we use high-resolution simulations of the isotope-enabled version of the regional weather and climate prediction model of the Consortium for Small-Scale Modelling (COSMO<span class="inline-formula"><sub>iso</sub></span>) to investigate predominant moisture transport pathways in the Canary Islands region in the eastern subtropical North Atlantic. Comparison of the simulated isotope signals with multi-platform isotope observations (aircraft, ground- and space-based remote sensing) from a field campaign in summer 2013 shows that COSMO<span class="inline-formula"><sub>iso</sub></span> can reproduce the observed variability of stable water vapour isotopes on timescales of hours to days, thus allowing us to study the mechanisms that control the subtropical free-tropospheric humidity. Changes in isotopic signals along backward trajectories from the Canary Islands region reveal the physical processes behind the synoptic-scale isotope variability. We identify four predominant moisture transport pathways of mid-tropospheric air, each with distinct isotopic signatures: </p><ol><li> <p id="d1e198">air parcels originating from the convective boundary layer of the Saharan heat low (SHL) – these are characterised by a homogeneous isotopic composition with a particularly high <span class="inline-formula"><i>δ</i>D</span> (median mid-tropospheric <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M4" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">122</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="ddf41a60fa08c188f8b6022f0b1d0971"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00001.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00001.png"/></svg:svg></span></span>), which results from dry convective mixing of low-level moisture of diverse origin advected into the SHL;</p></li><li> <p id="d1e233">air parcels originating from the free troposphere above the SHL – although experiencing the largest changes in humidity and <span class="inline-formula"><i>δ</i>D</span> during their subsidence over West Africa, these air parcels typically have lower <span class="inline-formula"><i>δ</i>D</span> values (median <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M7" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">148</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="5615454091bf1c5095c105b192a549fd"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00002.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00002.png"/></svg:svg></span></span>) than air parcels originating from the boundary layer of the SHL;</p></li><li> <p id="d1e279">air parcels originating from outside the SHL region, typically descending from tropical upper levels south of the SHL, which are often affected by moist convective injections from mesoscale convective systems in the Sahel – their isotopic composition is much less enriched in heavy isotopes (median <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M8" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">175</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="85a31394b7fce9c10b2f96be4f6cefe1"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00003.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00003.png"/></svg:svg></span></span>) than those from the SHL region;</p></li><li> <p id="d1e303">air parcels subsiding from the upper-level extratropical North Atlantic – this pathway leads to the driest and most depleted conditions (median <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M9" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">255</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="558bba7a1df0fcca52c1c7cca6be7938"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00004.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00004.png"/></svg:svg></span></span>) in the middle troposphere near the Canary Islands.</p></li></ol><p> The alternation of these transport pathways explains the observed high variability in humidity and <span class="inline-formula"><i>δ</i>D</span> on synoptic timescales to a large degree. We further show that the four different transport pathways are related to specific large-scale flow conditions. In particular, distinct differences in the location of the North African mid-level anticyclone and of extratropical Rossby wave patterns occur between the four transport pathways. Overall, this study demonstrates that the adopted Lagrangian isotope perspective enhances our understanding of air mass transport and mixing and offers a sound interpretation of the free-tropospheric variability of specific humidity and isotope composition on timescales of hours to days in contrasting atmospheric conditions over the eastern subtropical North Atlantic.</p>
format article
author F. Dahinden
F. Aemisegger
H. Wernli
M. Schneider
C. J. Diekmann
B. Ertl
P. Knippertz
M. Werner
S. Pfahl
author_facet F. Dahinden
F. Aemisegger
H. Wernli
M. Schneider
C. J. Diekmann
B. Ertl
P. Knippertz
M. Werner
S. Pfahl
author_sort F. Dahinden
title Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling
title_short Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling
title_full Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling
title_fullStr Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling
title_full_unstemmed Disentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling
title_sort disentangling different moisture transport pathways over the eastern subtropical north atlantic using multi-platform isotope observations and high-resolution numerical modelling
publisher Copernicus Publications
publishDate 2021
url https://doaj.org/article/20c76147d9644ddfaf7ef671937076d9
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AT hwernli disentanglingdifferentmoisturetransportpathwaysovertheeasternsubtropicalnorthatlanticusingmultiplatformisotopeobservationsandhighresolutionnumericalmodelling
AT mschneider disentanglingdifferentmoisturetransportpathwaysovertheeasternsubtropicalnorthatlanticusingmultiplatformisotopeobservationsandhighresolutionnumericalmodelling
AT cjdiekmann disentanglingdifferentmoisturetransportpathwaysovertheeasternsubtropicalnorthatlanticusingmultiplatformisotopeobservationsandhighresolutionnumericalmodelling
AT bertl disentanglingdifferentmoisturetransportpathwaysovertheeasternsubtropicalnorthatlanticusingmultiplatformisotopeobservationsandhighresolutionnumericalmodelling
AT pknippertz disentanglingdifferentmoisturetransportpathwaysovertheeasternsubtropicalnorthatlanticusingmultiplatformisotopeobservationsandhighresolutionnumericalmodelling
AT mwerner disentanglingdifferentmoisturetransportpathwaysovertheeasternsubtropicalnorthatlanticusingmultiplatformisotopeobservationsandhighresolutionnumericalmodelling
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spelling oai:doaj.org-article:20c76147d9644ddfaf7ef671937076d92021-11-08T10:43:20ZDisentangling different moisture transport pathways over the eastern subtropical North Atlantic using multi-platform isotope observations and high-resolution numerical modelling10.5194/acp-21-16319-20211680-73161680-7324https://doaj.org/article/20c76147d9644ddfaf7ef671937076d92021-11-01T00:00:00Zhttps://acp.copernicus.org/articles/21/16319/2021/acp-21-16319-2021.pdfhttps://doaj.org/toc/1680-7316https://doaj.org/toc/1680-7324<p>Due to its dryness, the subtropical free troposphere plays a critical role in the radiative balance of the Earth's climate system. But the complex interactions of the dynamical and physical processes controlling the variability in the moisture budget of this sensitive region of the subtropical atmosphere are still not fully understood. Stable water isotopes can provide important information about several of the latter processes, namely subsidence drying, turbulent mixing, and dry and moist convective moistening. In this study, we use high-resolution simulations of the isotope-enabled version of the regional weather and climate prediction model of the Consortium for Small-Scale Modelling (COSMO<span class="inline-formula"><sub>iso</sub></span>) to investigate predominant moisture transport pathways in the Canary Islands region in the eastern subtropical North Atlantic. Comparison of the simulated isotope signals with multi-platform isotope observations (aircraft, ground- and space-based remote sensing) from a field campaign in summer 2013 shows that COSMO<span class="inline-formula"><sub>iso</sub></span> can reproduce the observed variability of stable water vapour isotopes on timescales of hours to days, thus allowing us to study the mechanisms that control the subtropical free-tropospheric humidity. Changes in isotopic signals along backward trajectories from the Canary Islands region reveal the physical processes behind the synoptic-scale isotope variability. We identify four predominant moisture transport pathways of mid-tropospheric air, each with distinct isotopic signatures: </p><ol><li> <p id="d1e198">air parcels originating from the convective boundary layer of the Saharan heat low (SHL) – these are characterised by a homogeneous isotopic composition with a particularly high <span class="inline-formula"><i>δ</i>D</span> (median mid-tropospheric <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M4" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">122</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="ddf41a60fa08c188f8b6022f0b1d0971"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00001.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00001.png"/></svg:svg></span></span>), which results from dry convective mixing of low-level moisture of diverse origin advected into the SHL;</p></li><li> <p id="d1e233">air parcels originating from the free troposphere above the SHL – although experiencing the largest changes in humidity and <span class="inline-formula"><i>δ</i>D</span> during their subsidence over West Africa, these air parcels typically have lower <span class="inline-formula"><i>δ</i>D</span> values (median <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M7" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">148</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="5615454091bf1c5095c105b192a549fd"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00002.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00002.png"/></svg:svg></span></span>) than air parcels originating from the boundary layer of the SHL;</p></li><li> <p id="d1e279">air parcels originating from outside the SHL region, typically descending from tropical upper levels south of the SHL, which are often affected by moist convective injections from mesoscale convective systems in the Sahel – their isotopic composition is much less enriched in heavy isotopes (median <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M8" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">175</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="85a31394b7fce9c10b2f96be4f6cefe1"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00003.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00003.png"/></svg:svg></span></span>) than those from the SHL region;</p></li><li> <p id="d1e303">air parcels subsiding from the upper-level extratropical North Atlantic – this pathway leads to the driest and most depleted conditions (median <span class="inline-formula"><math xmlns="http://www.w3.org/1998/Math/MathML" id="M9" display="inline" overflow="scroll" dspmath="mathml"><mrow><mi mathvariant="italic">δ</mi><mrow class="chem"><mi mathvariant="normal">D</mi></mrow><mo>=</mo><mo>-</mo><mn mathvariant="normal">255</mn><mspace width="0.125em" linebreak="nobreak"/><mi mathvariant="normal">‰</mi></mrow></math><span><svg:svg xmlns:svg="http://www.w3.org/2000/svg" width="68pt" height="10pt" class="svg-formula" dspmath="mathimg" md5hash="558bba7a1df0fcca52c1c7cca6be7938"><svg:image xmlns:xlink="http://www.w3.org/1999/xlink" xlink:href="acp-21-16319-2021-ie00004.svg" width="68pt" height="10pt" src="acp-21-16319-2021-ie00004.png"/></svg:svg></span></span>) in the middle troposphere near the Canary Islands.</p></li></ol><p> The alternation of these transport pathways explains the observed high variability in humidity and <span class="inline-formula"><i>δ</i>D</span> on synoptic timescales to a large degree. We further show that the four different transport pathways are related to specific large-scale flow conditions. In particular, distinct differences in the location of the North African mid-level anticyclone and of extratropical Rossby wave patterns occur between the four transport pathways. Overall, this study demonstrates that the adopted Lagrangian isotope perspective enhances our understanding of air mass transport and mixing and offers a sound interpretation of the free-tropospheric variability of specific humidity and isotope composition on timescales of hours to days in contrasting atmospheric conditions over the eastern subtropical North Atlantic.</p>F. DahindenF. AemiseggerH. WernliM. SchneiderC. J. DiekmannB. ErtlP. KnippertzM. WernerS. PfahlCopernicus PublicationsarticlePhysicsQC1-999ChemistryQD1-999ENAtmospheric Chemistry and Physics, Vol 21, Pp 16319-16347 (2021)