Three-dimensional networks of superconducting NbSe2 flakes with nearly isotropic large upper critical field

Abstract Increasing the upper critical field H c2 in superconductors is one of the most significant requirements for superconducting applications. Two-dimensional (2D) noncentrosymmetric NbSe2 is a promising candidate because its pair breaking is protected by the spin-momentum locking effect, result...

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Autores principales: Togo Takahashi, Chisato Ando, Mitsufumi Saito, Yasumitsu Miyata, Yusuke Nakanishi, Jiang Pu, Taishi Takenobu
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/215361a0f8a7450d9539ce7546513833
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Sumario:Abstract Increasing the upper critical field H c2 in superconductors is one of the most significant requirements for superconducting applications. Two-dimensional (2D) noncentrosymmetric NbSe2 is a promising candidate because its pair breaking is protected by the spin-momentum locking effect, resulting in a giant in-plane H c2 (~50 T). However, the strong anisotropy of 2D NbSe2 suppresses the robustness of out-of-plane H c2 (<5 T). To overcome this issue, we propose a synthetic approach to produce superconducting NbSe2 films with a nearly isotropic large H c2. Scalable selenization methods are tailored to create 3D superconducting networks in which 2D NbSe2 flakes are vertically aligned to the substrates. The angle-resolved magneto-transports reveal enhanced H c2 values that exceed 20 T for arbitrary directions under externally applied magnetic fields. The isotropic nature of H c2 is attributed to the averaging intrinsic anisotropy of NbSe2 through 3D structured films, which was determined by X-ray diffraction measurements. The proposed synthetic approach will provide a new method for creating practical superconductors that are robust against magnetic fields.