Photodetector Based on CsPbBr<sub>3</sub>/Cs<sub>4</sub>PbBr<sub>6</sub> Composite Nanocrystals with High Detectivity

High-quality, all-inorganic CsPbBr<sub>3</sub>/Cs<sub>4</sub>PbBr<sub>6</sub> composite perovskite nanocrystals (NCs) were obtained with all-solution-processing at room temperature, and a photodetector (PD) with high detectivity was realized based on CsPbBr<sub...

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Autores principales: Yue Han, Rong Wen, Feng Zhang, Linlin Shi, Wenyan Wang, Ting Ji, Guohui Li, Yuying Hao, Lin Feng, Yanxia Cui
Formato: article
Lenguaje:EN
Publicado: MDPI AG 2021
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Acceso en línea:https://doaj.org/article/24b2fce106ed46b3b132438d575c0d48
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Sumario:High-quality, all-inorganic CsPbBr<sub>3</sub>/Cs<sub>4</sub>PbBr<sub>6</sub> composite perovskite nanocrystals (NCs) were obtained with all-solution-processing at room temperature, and a photodetector (PD) with high detectivity was realized based on CsPbBr<sub>3</sub>/Cs<sub>4</sub>PbBr<sub>6</sub> NCs. The detectivity (<i>D*</i>) of the proposed PD is 4.24 × 10<sup>12</sup> Jones under 532 nm illumination, which is among the highest levels for PDs based on all-inorganic perovskite NCs. In addition, a high linear dynamic range (LDR) of 115 dB under 1 V bias was also realized. Furthermore, the underlying mechanism for the enhanced performance of the proposed PD was discussed. Our work might promote the preparation of high-performance PDs based on dual-phase all-inorganic perovskite nanocrystals.