Unified model for singlet fission within a non-conjugated covalent pentacene dimer

Singlet fission is an important process occurring in solar cells, however the mechanism is not well understood. Here the authors reveal intermediates during singlet fission of a non-conjugated pentacene dimer, developing a single kinetic model to describe the data over seven temporal orders of magni...

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Autores principales: Bettina S. Basel, Johannes Zirzlmeier, Constantin Hetzer, Brian T. Phelan, Matthew D. Krzyaniak, S. Rajagopala Reddy, Pedro B. Coto, Noah E. Horwitz, Ryan M. Young, Fraser J. White, Frank Hampel, Timothy Clark, Michael Thoss, Rik R. Tykwinski, Michael R. Wasielewski, Dirk M. Guldi
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Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/24ef8610334242258a19ec1f33053b74
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spelling oai:doaj.org-article:24ef8610334242258a19ec1f33053b742021-12-02T15:38:31ZUnified model for singlet fission within a non-conjugated covalent pentacene dimer10.1038/ncomms151712041-1723https://doaj.org/article/24ef8610334242258a19ec1f33053b742017-05-01T00:00:00Zhttps://doi.org/10.1038/ncomms15171https://doaj.org/toc/2041-1723Singlet fission is an important process occurring in solar cells, however the mechanism is not well understood. Here the authors reveal intermediates during singlet fission of a non-conjugated pentacene dimer, developing a single kinetic model to describe the data over seven temporal orders of magnitude at room and cryogenic temperatures.Bettina S. BaselJohannes ZirzlmeierConstantin HetzerBrian T. PhelanMatthew D. KrzyaniakS. Rajagopala ReddyPedro B. CotoNoah E. HorwitzRyan M. YoungFraser J. WhiteFrank HampelTimothy ClarkMichael ThossRik R. TykwinskiMichael R. WasielewskiDirk M. GuldiNature PortfolioarticleScienceQENNature Communications, Vol 8, Iss 1, Pp 1-8 (2017)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Bettina S. Basel
Johannes Zirzlmeier
Constantin Hetzer
Brian T. Phelan
Matthew D. Krzyaniak
S. Rajagopala Reddy
Pedro B. Coto
Noah E. Horwitz
Ryan M. Young
Fraser J. White
Frank Hampel
Timothy Clark
Michael Thoss
Rik R. Tykwinski
Michael R. Wasielewski
Dirk M. Guldi
Unified model for singlet fission within a non-conjugated covalent pentacene dimer
description Singlet fission is an important process occurring in solar cells, however the mechanism is not well understood. Here the authors reveal intermediates during singlet fission of a non-conjugated pentacene dimer, developing a single kinetic model to describe the data over seven temporal orders of magnitude at room and cryogenic temperatures.
format article
author Bettina S. Basel
Johannes Zirzlmeier
Constantin Hetzer
Brian T. Phelan
Matthew D. Krzyaniak
S. Rajagopala Reddy
Pedro B. Coto
Noah E. Horwitz
Ryan M. Young
Fraser J. White
Frank Hampel
Timothy Clark
Michael Thoss
Rik R. Tykwinski
Michael R. Wasielewski
Dirk M. Guldi
author_facet Bettina S. Basel
Johannes Zirzlmeier
Constantin Hetzer
Brian T. Phelan
Matthew D. Krzyaniak
S. Rajagopala Reddy
Pedro B. Coto
Noah E. Horwitz
Ryan M. Young
Fraser J. White
Frank Hampel
Timothy Clark
Michael Thoss
Rik R. Tykwinski
Michael R. Wasielewski
Dirk M. Guldi
author_sort Bettina S. Basel
title Unified model for singlet fission within a non-conjugated covalent pentacene dimer
title_short Unified model for singlet fission within a non-conjugated covalent pentacene dimer
title_full Unified model for singlet fission within a non-conjugated covalent pentacene dimer
title_fullStr Unified model for singlet fission within a non-conjugated covalent pentacene dimer
title_full_unstemmed Unified model for singlet fission within a non-conjugated covalent pentacene dimer
title_sort unified model for singlet fission within a non-conjugated covalent pentacene dimer
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/24ef8610334242258a19ec1f33053b74
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