Crystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed
Abstract ZnO-based ultraviolet (UV) photodetector can be easily fabricated by using sol–gel spin-coating method, however, the crystallization of amorphous state ZnO thin films is necessary to fabricate high performance UV photodetector. Thus, we devised a thermal dissipation annealing (TDA) method i...
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2021
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oai:doaj.org-article:263d641cc17b4e548e86e978012e9dcf2021-12-02T14:12:45ZCrystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed10.1038/s41598-020-79849-z2045-2322https://doaj.org/article/263d641cc17b4e548e86e978012e9dcf2021-01-01T00:00:00Zhttps://doi.org/10.1038/s41598-020-79849-zhttps://doaj.org/toc/2045-2322Abstract ZnO-based ultraviolet (UV) photodetector can be easily fabricated by using sol–gel spin-coating method, however, the crystallization of amorphous state ZnO thin films is necessary to fabricate high performance UV photodetector. Thus, we devised a thermal dissipation annealing (TDA) method in which the heat transfer to the ZnO thin films can be synchronized with the heat release from the substrate. It was found that sol–gel spin-coated ZnO thin films can be crystallized through the mobility difference of ZnO molecules placed at the surface of ZnO thin films. Also, UV photodetector based on ZnO thin films annealed with the TDA method exhibited faster rise and decay time constant (τr = 35 ms and τd = 73 ms, respectively), a higher on/off current ratio, and reproducible photocurrent characteristics compared to that of the ZnO thin films annealed by using furnace and IR lamp. Therefore, these results indicated that the TDA method is a feasible alternative route for the fabrication of ZnO based high performance optoelectronic devices.Dongwan KimJae-Young LeemNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-10 (2021) |
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Medicine R Science Q Dongwan Kim Jae-Young Leem Crystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed |
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Abstract ZnO-based ultraviolet (UV) photodetector can be easily fabricated by using sol–gel spin-coating method, however, the crystallization of amorphous state ZnO thin films is necessary to fabricate high performance UV photodetector. Thus, we devised a thermal dissipation annealing (TDA) method in which the heat transfer to the ZnO thin films can be synchronized with the heat release from the substrate. It was found that sol–gel spin-coated ZnO thin films can be crystallized through the mobility difference of ZnO molecules placed at the surface of ZnO thin films. Also, UV photodetector based on ZnO thin films annealed with the TDA method exhibited faster rise and decay time constant (τr = 35 ms and τd = 73 ms, respectively), a higher on/off current ratio, and reproducible photocurrent characteristics compared to that of the ZnO thin films annealed by using furnace and IR lamp. Therefore, these results indicated that the TDA method is a feasible alternative route for the fabrication of ZnO based high performance optoelectronic devices. |
format |
article |
author |
Dongwan Kim Jae-Young Leem |
author_facet |
Dongwan Kim Jae-Young Leem |
author_sort |
Dongwan Kim |
title |
Crystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed |
title_short |
Crystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed |
title_full |
Crystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed |
title_fullStr |
Crystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed |
title_full_unstemmed |
Crystallization of ZnO thin films via thermal dissipation annealing method for high-performance UV photodetector with ultrahigh response speed |
title_sort |
crystallization of zno thin films via thermal dissipation annealing method for high-performance uv photodetector with ultrahigh response speed |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/263d641cc17b4e548e86e978012e9dcf |
work_keys_str_mv |
AT dongwankim crystallizationofznothinfilmsviathermaldissipationannealingmethodforhighperformanceuvphotodetectorwithultrahighresponsespeed AT jaeyoungleem crystallizationofznothinfilmsviathermaldissipationannealingmethodforhighperformanceuvphotodetectorwithultrahighresponsespeed |
_version_ |
1718391775176949760 |