Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser

The nonlinear optical properties and ultrafast dynamics process of Au@Ag coreshell nanospheres (NSs) are reported in this paper. We researched the optical nonlinear absorption property of Au@Ag coreshell NSs excited by 800 nm laser at different energies by open-aperture Z-scan technology. The experi...

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Autores principales: Jun Wang, Jijuan Jiang, Yabin Shao, Wenzhi Wu, Degui Kong, Yachen Gao
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Publicado: AIP Publishing LLC 2021
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Acceso en línea:https://doaj.org/article/267b5d32b10f4cef9db8f9881be36105
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spelling oai:doaj.org-article:267b5d32b10f4cef9db8f9881be361052021-12-01T18:52:06ZNonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser2158-322610.1063/5.0067588https://doaj.org/article/267b5d32b10f4cef9db8f9881be361052021-11-01T00:00:00Zhttp://dx.doi.org/10.1063/5.0067588https://doaj.org/toc/2158-3226The nonlinear optical properties and ultrafast dynamics process of Au@Ag coreshell nanospheres (NSs) are reported in this paper. We researched the optical nonlinear absorption property of Au@Ag coreshell NSs excited by 800 nm laser at different energies by open-aperture Z-scan technology. The experimental results demonstrated that the Au@Ag coreshell NSs exhibited two-phone absorption (TPA) behavior, the degree of which was intensity-dependent. The TPA coefficients of Au@Ag coreshell NSs excited by different energies were obtained by fitting. By using pump-probe technology, we studied the ultrafast dynamics process of Au@Ag coreshell NSs. The results indicated that the relaxation process contained a fast and a slow process, which depended strongly on the laser intensity. By numerical fitting, we got the relaxation times of the sample excited at different laser powers.Jun WangJijuan JiangYabin ShaoWenzhi WuDegui KongYachen GaoAIP Publishing LLCarticlePhysicsQC1-999ENAIP Advances, Vol 11, Iss 11, Pp 115109-115109-5 (2021)
institution DOAJ
collection DOAJ
language EN
topic Physics
QC1-999
spellingShingle Physics
QC1-999
Jun Wang
Jijuan Jiang
Yabin Shao
Wenzhi Wu
Degui Kong
Yachen Gao
Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser
description The nonlinear optical properties and ultrafast dynamics process of Au@Ag coreshell nanospheres (NSs) are reported in this paper. We researched the optical nonlinear absorption property of Au@Ag coreshell NSs excited by 800 nm laser at different energies by open-aperture Z-scan technology. The experimental results demonstrated that the Au@Ag coreshell NSs exhibited two-phone absorption (TPA) behavior, the degree of which was intensity-dependent. The TPA coefficients of Au@Ag coreshell NSs excited by different energies were obtained by fitting. By using pump-probe technology, we studied the ultrafast dynamics process of Au@Ag coreshell NSs. The results indicated that the relaxation process contained a fast and a slow process, which depended strongly on the laser intensity. By numerical fitting, we got the relaxation times of the sample excited at different laser powers.
format article
author Jun Wang
Jijuan Jiang
Yabin Shao
Wenzhi Wu
Degui Kong
Yachen Gao
author_facet Jun Wang
Jijuan Jiang
Yabin Shao
Wenzhi Wu
Degui Kong
Yachen Gao
author_sort Jun Wang
title Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser
title_short Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser
title_full Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser
title_fullStr Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser
title_full_unstemmed Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser
title_sort nonlinear optical properties of au@ag coreshell nanospheres excited by femtosecond laser
publisher AIP Publishing LLC
publishDate 2021
url https://doaj.org/article/267b5d32b10f4cef9db8f9881be36105
work_keys_str_mv AT junwang nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser
AT jijuanjiang nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser
AT yabinshao nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser
AT wenzhiwu nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser
AT deguikong nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser
AT yachengao nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser
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