Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser
The nonlinear optical properties and ultrafast dynamics process of Au@Ag coreshell nanospheres (NSs) are reported in this paper. We researched the optical nonlinear absorption property of Au@Ag coreshell NSs excited by 800 nm laser at different energies by open-aperture Z-scan technology. The experi...
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2021
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oai:doaj.org-article:267b5d32b10f4cef9db8f9881be361052021-12-01T18:52:06ZNonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser2158-322610.1063/5.0067588https://doaj.org/article/267b5d32b10f4cef9db8f9881be361052021-11-01T00:00:00Zhttp://dx.doi.org/10.1063/5.0067588https://doaj.org/toc/2158-3226The nonlinear optical properties and ultrafast dynamics process of Au@Ag coreshell nanospheres (NSs) are reported in this paper. We researched the optical nonlinear absorption property of Au@Ag coreshell NSs excited by 800 nm laser at different energies by open-aperture Z-scan technology. The experimental results demonstrated that the Au@Ag coreshell NSs exhibited two-phone absorption (TPA) behavior, the degree of which was intensity-dependent. The TPA coefficients of Au@Ag coreshell NSs excited by different energies were obtained by fitting. By using pump-probe technology, we studied the ultrafast dynamics process of Au@Ag coreshell NSs. The results indicated that the relaxation process contained a fast and a slow process, which depended strongly on the laser intensity. By numerical fitting, we got the relaxation times of the sample excited at different laser powers.Jun WangJijuan JiangYabin ShaoWenzhi WuDegui KongYachen GaoAIP Publishing LLCarticlePhysicsQC1-999ENAIP Advances, Vol 11, Iss 11, Pp 115109-115109-5 (2021) |
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Physics QC1-999 |
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Physics QC1-999 Jun Wang Jijuan Jiang Yabin Shao Wenzhi Wu Degui Kong Yachen Gao Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser |
description |
The nonlinear optical properties and ultrafast dynamics process of Au@Ag coreshell nanospheres (NSs) are reported in this paper. We researched the optical nonlinear absorption property of Au@Ag coreshell NSs excited by 800 nm laser at different energies by open-aperture Z-scan technology. The experimental results demonstrated that the Au@Ag coreshell NSs exhibited two-phone absorption (TPA) behavior, the degree of which was intensity-dependent. The TPA coefficients of Au@Ag coreshell NSs excited by different energies were obtained by fitting. By using pump-probe technology, we studied the ultrafast dynamics process of Au@Ag coreshell NSs. The results indicated that the relaxation process contained a fast and a slow process, which depended strongly on the laser intensity. By numerical fitting, we got the relaxation times of the sample excited at different laser powers. |
format |
article |
author |
Jun Wang Jijuan Jiang Yabin Shao Wenzhi Wu Degui Kong Yachen Gao |
author_facet |
Jun Wang Jijuan Jiang Yabin Shao Wenzhi Wu Degui Kong Yachen Gao |
author_sort |
Jun Wang |
title |
Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser |
title_short |
Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser |
title_full |
Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser |
title_fullStr |
Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser |
title_full_unstemmed |
Nonlinear optical properties of Au@Ag coreshell nanospheres excited by femtosecond laser |
title_sort |
nonlinear optical properties of au@ag coreshell nanospheres excited by femtosecond laser |
publisher |
AIP Publishing LLC |
publishDate |
2021 |
url |
https://doaj.org/article/267b5d32b10f4cef9db8f9881be36105 |
work_keys_str_mv |
AT junwang nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser AT jijuanjiang nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser AT yabinshao nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser AT wenzhiwu nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser AT deguikong nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser AT yachengao nonlinearopticalpropertiesofauagcoreshellnanospheresexcitedbyfemtosecondlaser |
_version_ |
1718404680250294272 |