Structural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation

The uncontrolled and unethical release of pharmaceutical contaminants into aquatic sources have severe adversities, including the possible emergence of antimicrobial-resistant bacteria. Photocatalysis utilizing semiconductor heterostructures is a greener and sustainable option for the effective degr...

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Autores principales: P. Suyana, Priyanka Ganguly, Balagopal N. Nair, Suresh C. Pillai, U. S. Hareesh
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Publicado: Elsevier 2021
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Acceso en línea:https://doaj.org/article/26ad4713b5ab4ebbab2bec1c1502ce39
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spelling oai:doaj.org-article:26ad4713b5ab4ebbab2bec1c1502ce392021-11-18T04:52:47ZStructural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation2666-821110.1016/j.ceja.2021.100148https://doaj.org/article/26ad4713b5ab4ebbab2bec1c1502ce392021-11-01T00:00:00Zhttp://www.sciencedirect.com/science/article/pii/S2666821121000648https://doaj.org/toc/2666-8211The uncontrolled and unethical release of pharmaceutical contaminants into aquatic sources have severe adversities, including the possible emergence of antimicrobial-resistant bacteria. Photocatalysis utilizing semiconductor heterostructures is a greener and sustainable option for the effective degradation of organic contaminants into relatively harmless by-products. Visible/sunlight active graphitic carbon nitride based photocatalysts have been explored for antibiotic degradation (Tetracycline, Doxycycline, Oxytetracycline, Sulfamethoxazole, Amoxicillin) owing to their excellent chemical/thermal stability, tunable photophysical properties and facile methods of synthesis. The properties were further enhanced by heterostructure formation with other compatible semiconductors, elemental/molecular doping and through the creation of hierarchically porous structures. Moreover, nanocomposite formation with high surface area porous frameworks induces adsorptive photocatalysis imparting bifunctionality and alleviating secondary remediation measures for regeneration of the catalysts. The review summarizes the efforts in developing C3N4 based systems for the effective degradation of various antibiotics. Finally, an outlook on essential improvements is forecasted.P. SuyanaPriyanka GangulyBalagopal N. NairSuresh C. PillaiU. S. HareeshElsevierarticleAntibiotic wasteCircular economyPhotocatalysisGraphitic carbon nitrideWaste to energySurface modificationChemical engineeringTP155-156ENChemical Engineering Journal Advances, Vol 8, Iss , Pp 100148- (2021)
institution DOAJ
collection DOAJ
language EN
topic Antibiotic waste
Circular economy
Photocatalysis
Graphitic carbon nitride
Waste to energy
Surface modification
Chemical engineering
TP155-156
spellingShingle Antibiotic waste
Circular economy
Photocatalysis
Graphitic carbon nitride
Waste to energy
Surface modification
Chemical engineering
TP155-156
P. Suyana
Priyanka Ganguly
Balagopal N. Nair
Suresh C. Pillai
U. S. Hareesh
Structural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation
description The uncontrolled and unethical release of pharmaceutical contaminants into aquatic sources have severe adversities, including the possible emergence of antimicrobial-resistant bacteria. Photocatalysis utilizing semiconductor heterostructures is a greener and sustainable option for the effective degradation of organic contaminants into relatively harmless by-products. Visible/sunlight active graphitic carbon nitride based photocatalysts have been explored for antibiotic degradation (Tetracycline, Doxycycline, Oxytetracycline, Sulfamethoxazole, Amoxicillin) owing to their excellent chemical/thermal stability, tunable photophysical properties and facile methods of synthesis. The properties were further enhanced by heterostructure formation with other compatible semiconductors, elemental/molecular doping and through the creation of hierarchically porous structures. Moreover, nanocomposite formation with high surface area porous frameworks induces adsorptive photocatalysis imparting bifunctionality and alleviating secondary remediation measures for regeneration of the catalysts. The review summarizes the efforts in developing C3N4 based systems for the effective degradation of various antibiotics. Finally, an outlook on essential improvements is forecasted.
format article
author P. Suyana
Priyanka Ganguly
Balagopal N. Nair
Suresh C. Pillai
U. S. Hareesh
author_facet P. Suyana
Priyanka Ganguly
Balagopal N. Nair
Suresh C. Pillai
U. S. Hareesh
author_sort P. Suyana
title Structural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation
title_short Structural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation
title_full Structural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation
title_fullStr Structural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation
title_full_unstemmed Structural and compositional tuning in g-C3N4 based systems for photocatalytic antibiotic degradation
title_sort structural and compositional tuning in g-c3n4 based systems for photocatalytic antibiotic degradation
publisher Elsevier
publishDate 2021
url https://doaj.org/article/26ad4713b5ab4ebbab2bec1c1502ce39
work_keys_str_mv AT psuyana structuralandcompositionaltuningingc3n4basedsystemsforphotocatalyticantibioticdegradation
AT priyankaganguly structuralandcompositionaltuningingc3n4basedsystemsforphotocatalyticantibioticdegradation
AT balagopalnnair structuralandcompositionaltuningingc3n4basedsystemsforphotocatalyticantibioticdegradation
AT sureshcpillai structuralandcompositionaltuningingc3n4basedsystemsforphotocatalyticantibioticdegradation
AT ushareesh structuralandcompositionaltuningingc3n4basedsystemsforphotocatalyticantibioticdegradation
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