In situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity

In situ tuning of the electronic structure of active sites is a long-standing challenge. Here, the authors report an approach to tune the electronic structure of cobalt species during the styrene epoxidation reaction by the introduction of controllable hydrogen spillover for enhanced selectivity.

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Autores principales: Mi Xiong, Zhe Gao, Peng Zhao, Guofu Wang, Wenjun Yan, Shuangfeng Xing, Pengfei Wang, Jingyuan Ma, Zheng Jiang, Xingchen Liu, Jiping Ma, Jie Xu, Yong Qin
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Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/26b8d51b255e4cacbbc5790f1e11d737
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spelling oai:doaj.org-article:26b8d51b255e4cacbbc5790f1e11d7372021-12-02T15:14:48ZIn situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity10.1038/s41467-020-18567-62041-1723https://doaj.org/article/26b8d51b255e4cacbbc5790f1e11d7372020-09-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-18567-6https://doaj.org/toc/2041-1723In situ tuning of the electronic structure of active sites is a long-standing challenge. Here, the authors report an approach to tune the electronic structure of cobalt species during the styrene epoxidation reaction by the introduction of controllable hydrogen spillover for enhanced selectivity.Mi XiongZhe GaoPeng ZhaoGuofu WangWenjun YanShuangfeng XingPengfei WangJingyuan MaZheng JiangXingchen LiuJiping MaJie XuYong QinNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-10 (2020)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Mi Xiong
Zhe Gao
Peng Zhao
Guofu Wang
Wenjun Yan
Shuangfeng Xing
Pengfei Wang
Jingyuan Ma
Zheng Jiang
Xingchen Liu
Jiping Ma
Jie Xu
Yong Qin
In situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity
description In situ tuning of the electronic structure of active sites is a long-standing challenge. Here, the authors report an approach to tune the electronic structure of cobalt species during the styrene epoxidation reaction by the introduction of controllable hydrogen spillover for enhanced selectivity.
format article
author Mi Xiong
Zhe Gao
Peng Zhao
Guofu Wang
Wenjun Yan
Shuangfeng Xing
Pengfei Wang
Jingyuan Ma
Zheng Jiang
Xingchen Liu
Jiping Ma
Jie Xu
Yong Qin
author_facet Mi Xiong
Zhe Gao
Peng Zhao
Guofu Wang
Wenjun Yan
Shuangfeng Xing
Pengfei Wang
Jingyuan Ma
Zheng Jiang
Xingchen Liu
Jiping Ma
Jie Xu
Yong Qin
author_sort Mi Xiong
title In situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity
title_short In situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity
title_full In situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity
title_fullStr In situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity
title_full_unstemmed In situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity
title_sort in situ tuning of electronic structure of catalysts using controllable hydrogen spillover for enhanced selectivity
publisher Nature Portfolio
publishDate 2020
url https://doaj.org/article/26b8d51b255e4cacbbc5790f1e11d737
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