Optimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method

The present work demonstrated preparation of coal-based electrode materials (CEM)-derived low-rank coal for simultaneous removal of ammonia nitrogen (NH3-N) and chemical oxygen demand (COD) from coking wastewater by a three-dimensional electrode system (3DES). The influence of important parameters i...

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Autores principales: Su Ting, Gao Wenwen, Xing Xiangdong, Lan Xinzhe, Song Yonghui
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Lenguaje:EN
Publicado: De Gruyter 2021
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Acceso en línea:https://doaj.org/article/271c09b2f20b43afbf8b7fdc1c134e8f
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spelling oai:doaj.org-article:271c09b2f20b43afbf8b7fdc1c134e8f2021-12-05T14:10:50ZOptimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method2191-955010.1515/gps-2021-0072https://doaj.org/article/271c09b2f20b43afbf8b7fdc1c134e8f2021-11-01T00:00:00Zhttps://doi.org/10.1515/gps-2021-0072https://doaj.org/toc/2191-9550The present work demonstrated preparation of coal-based electrode materials (CEM)-derived low-rank coal for simultaneous removal of ammonia nitrogen (NH3-N) and chemical oxygen demand (COD) from coking wastewater by a three-dimensional electrode system (3DES). The influence of important parameters in 3DES such as processing time, applied voltage, electrode plate spacing, mass of commercially activated carbon (CAC), and initial pH were investigated. Based on the central composite design, the response surface method (RSM) was employed in order to optimize the variable parameters in removal process of pollutants. From the analysis of RSM, the optimum conditions for 3DES were 4.5 h of processing time, 5.5 V of applied voltage, 17 mm electrode plate spacing, 4.5 g CAC, and pH of 3 with higher simultaneous removal rate of COD (74.20%) and NH3-N (51.48%). Besides, the content of N element (4.9%) and N containing groups were traced by SEM-EDS and FTIR analysis in order to verify the removal effect. The experiment results showed the capability of CEM for electrode system removal of pollutants from coking wastewater and obtained considerable simultaneous removal rate of NH3-N and COD.Su TingGao WenwenXing XiangdongLan XinzheSong YonghuiDe Gruyterarticlenh3-n and codsimultaneous removal ratethree-dimensional electrode systemcoal-based electrode materialsresponse surface methodChemistryQD1-999ENGreen Processing and Synthesis, Vol 10, Iss 1, Pp 756-767 (2021)
institution DOAJ
collection DOAJ
language EN
topic nh3-n and cod
simultaneous removal rate
three-dimensional electrode system
coal-based electrode materials
response surface method
Chemistry
QD1-999
spellingShingle nh3-n and cod
simultaneous removal rate
three-dimensional electrode system
coal-based electrode materials
response surface method
Chemistry
QD1-999
Su Ting
Gao Wenwen
Xing Xiangdong
Lan Xinzhe
Song Yonghui
Optimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method
description The present work demonstrated preparation of coal-based electrode materials (CEM)-derived low-rank coal for simultaneous removal of ammonia nitrogen (NH3-N) and chemical oxygen demand (COD) from coking wastewater by a three-dimensional electrode system (3DES). The influence of important parameters in 3DES such as processing time, applied voltage, electrode plate spacing, mass of commercially activated carbon (CAC), and initial pH were investigated. Based on the central composite design, the response surface method (RSM) was employed in order to optimize the variable parameters in removal process of pollutants. From the analysis of RSM, the optimum conditions for 3DES were 4.5 h of processing time, 5.5 V of applied voltage, 17 mm electrode plate spacing, 4.5 g CAC, and pH of 3 with higher simultaneous removal rate of COD (74.20%) and NH3-N (51.48%). Besides, the content of N element (4.9%) and N containing groups were traced by SEM-EDS and FTIR analysis in order to verify the removal effect. The experiment results showed the capability of CEM for electrode system removal of pollutants from coking wastewater and obtained considerable simultaneous removal rate of NH3-N and COD.
format article
author Su Ting
Gao Wenwen
Xing Xiangdong
Lan Xinzhe
Song Yonghui
author_facet Su Ting
Gao Wenwen
Xing Xiangdong
Lan Xinzhe
Song Yonghui
author_sort Su Ting
title Optimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method
title_short Optimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method
title_full Optimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method
title_fullStr Optimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method
title_full_unstemmed Optimization for simultaneous removal of NH3-N and COD from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by RSM method
title_sort optimization for simultaneous removal of nh3-n and cod from coking wastewater via a three-dimensional electrode system with coal-based electrode materials by rsm method
publisher De Gruyter
publishDate 2021
url https://doaj.org/article/271c09b2f20b43afbf8b7fdc1c134e8f
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AT xingxiangdong optimizationforsimultaneousremovalofnh3nandcodfromcokingwastewaterviaathreedimensionalelectrodesystemwithcoalbasedelectrodematerialsbyrsmmethod
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