Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides

Proton-coupled electron transfer (PCET) has been observed in chemical, energy, and biological transformation processes. Here we demonstrate that the rate of PCET and oxygen evolution reaction can be dramatically enhanced by tuning crystal orientation and the correlated proton diffusion.

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Autores principales:	Yunmin Zhu, Zuyun He, YongMan Choi, Huijun Chen, Xiaobao Li, Bote Zhao, Yi Yu, Hui Zhang, Kelsey A. Stoerzinger, Zhenxing Feng, Yan Chen, Meilin Liu
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2020
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/285195b73e7349dbb118dd46d7cbf9a1
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spelling	oai:doaj.org-article:285195b73e7349dbb118dd46d7cbf9a12021-12-02T19:02:36ZTuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides10.1038/s41467-020-17657-92041-1723https://doaj.org/article/285195b73e7349dbb118dd46d7cbf9a12020-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-17657-9https://doaj.org/toc/2041-1723Proton-coupled electron transfer (PCET) has been observed in chemical, energy, and biological transformation processes. Here we demonstrate that the rate of PCET and oxygen evolution reaction can be dramatically enhanced by tuning crystal orientation and the correlated proton diffusion.Yunmin ZhuZuyun HeYongMan ChoiHuijun ChenXiaobao LiBote ZhaoYi YuHui ZhangKelsey A. StoerzingerZhenxing FengYan ChenMeilin LiuNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-10 (2020)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Yunmin Zhu Zuyun He YongMan Choi Huijun Chen Xiaobao Li Bote Zhao Yi Yu Hui Zhang Kelsey A. Stoerzinger Zhenxing Feng Yan Chen Meilin Liu Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides
description	Proton-coupled electron transfer (PCET) has been observed in chemical, energy, and biological transformation processes. Here we demonstrate that the rate of PCET and oxygen evolution reaction can be dramatically enhanced by tuning crystal orientation and the correlated proton diffusion.
format	article
author	Yunmin Zhu Zuyun He YongMan Choi Huijun Chen Xiaobao Li Bote Zhao Yi Yu Hui Zhang Kelsey A. Stoerzinger Zhenxing Feng Yan Chen Meilin Liu
author_facet	Yunmin Zhu Zuyun He YongMan Choi Huijun Chen Xiaobao Li Bote Zhao Yi Yu Hui Zhang Kelsey A. Stoerzinger Zhenxing Feng Yan Chen Meilin Liu
author_sort	Yunmin Zhu
title	Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides
title_short	Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides
title_full	Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides
title_fullStr	Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides
title_full_unstemmed	Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides
title_sort	tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides
publisher	Nature Portfolio
publishDate	2020
url	https://doaj.org/article/285195b73e7349dbb118dd46d7cbf9a1
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Tuning proton-coupled electron transfer by crystal orientation for efficient water oxidization on double perovskite oxides

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