Long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics

Anharmonic ultrafast structural dynamics are expected in lead halide perovskites due to their soft nature. Here Rivett et al. show that these dynamics lead to picosecond-long polarization anisotropy of photo-carriers in several halide perovskites, orders of magnitude slower than in conventional semi...

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Autores principales: Jasmine P. H. Rivett, Liang Z. Tan, Michael B. Price, Sean A. Bourelle, Nathaniel J. L. K. Davis, James Xiao, Yatao Zou, Rox Middleton, Baoquan Sun, Andrew M. Rappe, Dan Credgington, Felix Deschler
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Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/288a2808402a4166a2d6eb37f03e50dd
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spelling oai:doaj.org-article:288a2808402a4166a2d6eb37f03e50dd2021-12-02T17:32:18ZLong-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics10.1038/s41467-018-06009-32041-1723https://doaj.org/article/288a2808402a4166a2d6eb37f03e50dd2018-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-06009-3https://doaj.org/toc/2041-1723Anharmonic ultrafast structural dynamics are expected in lead halide perovskites due to their soft nature. Here Rivett et al. show that these dynamics lead to picosecond-long polarization anisotropy of photo-carriers in several halide perovskites, orders of magnitude slower than in conventional semiconductors.Jasmine P. H. RivettLiang Z. TanMichael B. PriceSean A. BourelleNathaniel J. L. K. DavisJames XiaoYatao ZouRox MiddletonBaoquan SunAndrew M. RappeDan CredgingtonFelix DeschlerNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-8 (2018)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Jasmine P. H. Rivett
Liang Z. Tan
Michael B. Price
Sean A. Bourelle
Nathaniel J. L. K. Davis
James Xiao
Yatao Zou
Rox Middleton
Baoquan Sun
Andrew M. Rappe
Dan Credgington
Felix Deschler
Long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics
description Anharmonic ultrafast structural dynamics are expected in lead halide perovskites due to their soft nature. Here Rivett et al. show that these dynamics lead to picosecond-long polarization anisotropy of photo-carriers in several halide perovskites, orders of magnitude slower than in conventional semiconductors.
format article
author Jasmine P. H. Rivett
Liang Z. Tan
Michael B. Price
Sean A. Bourelle
Nathaniel J. L. K. Davis
James Xiao
Yatao Zou
Rox Middleton
Baoquan Sun
Andrew M. Rappe
Dan Credgington
Felix Deschler
author_facet Jasmine P. H. Rivett
Liang Z. Tan
Michael B. Price
Sean A. Bourelle
Nathaniel J. L. K. Davis
James Xiao
Yatao Zou
Rox Middleton
Baoquan Sun
Andrew M. Rappe
Dan Credgington
Felix Deschler
author_sort Jasmine P. H. Rivett
title Long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics
title_short Long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics
title_full Long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics
title_fullStr Long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics
title_full_unstemmed Long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics
title_sort long-lived polarization memory in the electronic states of lead-halide perovskites from local structural dynamics
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/288a2808402a4166a2d6eb37f03e50dd
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