Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach

Abstract Micropatterning of transition metal dichalcogenide (TMDC) ultrathin-films and monolayers has been demonstrated by various multi-step approaches. However, directly achieving a patterned growth of TMDC films is still considered to be challenging. Here, we report a solution-based approach for...

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Autores principales: Devendra Pareek, Kathryna G. Roach, Marco A. Gonzalez, Lukas Büsing, Jürgen Parisi, Levent Gütay, Sascha Schäfer
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Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/28e53fea417c464a92ac02e44ad933d8
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spelling oai:doaj.org-article:28e53fea417c464a92ac02e44ad933d82021-12-02T15:39:41ZMicro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach10.1038/s41598-021-93278-62045-2322https://doaj.org/article/28e53fea417c464a92ac02e44ad933d82021-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-93278-6https://doaj.org/toc/2045-2322Abstract Micropatterning of transition metal dichalcogenide (TMDC) ultrathin-films and monolayers has been demonstrated by various multi-step approaches. However, directly achieving a patterned growth of TMDC films is still considered to be challenging. Here, we report a solution-based approach for the synthesis of patterned MoS2 layers by dragging a precursor solution droplet with variable velocities across a substrate. Utilizing the pronounced shearing velocity dependence in a Landau-Levich deposition regime, MoS2 films with a spatially modulated thickness with alternating mono/bi- and few-layer regions are obtained after precursor annealing. Generally, the presented facile methodology allows for the direct preparation of micro-structured functional materials, extendable to other TMDC materials and even van der Waals heterostructures.Devendra PareekKathryna G. RoachMarco A. GonzalezLukas BüsingJürgen ParisiLevent GütaySascha SchäferNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-7 (2021)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Devendra Pareek
Kathryna G. Roach
Marco A. Gonzalez
Lukas Büsing
Jürgen Parisi
Levent Gütay
Sascha Schäfer
Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach
description Abstract Micropatterning of transition metal dichalcogenide (TMDC) ultrathin-films and monolayers has been demonstrated by various multi-step approaches. However, directly achieving a patterned growth of TMDC films is still considered to be challenging. Here, we report a solution-based approach for the synthesis of patterned MoS2 layers by dragging a precursor solution droplet with variable velocities across a substrate. Utilizing the pronounced shearing velocity dependence in a Landau-Levich deposition regime, MoS2 films with a spatially modulated thickness with alternating mono/bi- and few-layer regions are obtained after precursor annealing. Generally, the presented facile methodology allows for the direct preparation of micro-structured functional materials, extendable to other TMDC materials and even van der Waals heterostructures.
format article
author Devendra Pareek
Kathryna G. Roach
Marco A. Gonzalez
Lukas Büsing
Jürgen Parisi
Levent Gütay
Sascha Schäfer
author_facet Devendra Pareek
Kathryna G. Roach
Marco A. Gonzalez
Lukas Büsing
Jürgen Parisi
Levent Gütay
Sascha Schäfer
author_sort Devendra Pareek
title Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach
title_short Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach
title_full Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach
title_fullStr Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach
title_full_unstemmed Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach
title_sort micro-patterned deposition of mos2 ultrathin-films by a controlled droplet dragging approach
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/28e53fea417c464a92ac02e44ad933d8
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