Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach
Abstract Micropatterning of transition metal dichalcogenide (TMDC) ultrathin-films and monolayers has been demonstrated by various multi-step approaches. However, directly achieving a patterned growth of TMDC films is still considered to be challenging. Here, we report a solution-based approach for...
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Nature Portfolio
2021
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oai:doaj.org-article:28e53fea417c464a92ac02e44ad933d82021-12-02T15:39:41ZMicro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach10.1038/s41598-021-93278-62045-2322https://doaj.org/article/28e53fea417c464a92ac02e44ad933d82021-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-93278-6https://doaj.org/toc/2045-2322Abstract Micropatterning of transition metal dichalcogenide (TMDC) ultrathin-films and monolayers has been demonstrated by various multi-step approaches. However, directly achieving a patterned growth of TMDC films is still considered to be challenging. Here, we report a solution-based approach for the synthesis of patterned MoS2 layers by dragging a precursor solution droplet with variable velocities across a substrate. Utilizing the pronounced shearing velocity dependence in a Landau-Levich deposition regime, MoS2 films with a spatially modulated thickness with alternating mono/bi- and few-layer regions are obtained after precursor annealing. Generally, the presented facile methodology allows for the direct preparation of micro-structured functional materials, extendable to other TMDC materials and even van der Waals heterostructures.Devendra PareekKathryna G. RoachMarco A. GonzalezLukas BüsingJürgen ParisiLevent GütaySascha SchäferNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-7 (2021) |
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Medicine R Science Q Devendra Pareek Kathryna G. Roach Marco A. Gonzalez Lukas Büsing Jürgen Parisi Levent Gütay Sascha Schäfer Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach |
description |
Abstract Micropatterning of transition metal dichalcogenide (TMDC) ultrathin-films and monolayers has been demonstrated by various multi-step approaches. However, directly achieving a patterned growth of TMDC films is still considered to be challenging. Here, we report a solution-based approach for the synthesis of patterned MoS2 layers by dragging a precursor solution droplet with variable velocities across a substrate. Utilizing the pronounced shearing velocity dependence in a Landau-Levich deposition regime, MoS2 films with a spatially modulated thickness with alternating mono/bi- and few-layer regions are obtained after precursor annealing. Generally, the presented facile methodology allows for the direct preparation of micro-structured functional materials, extendable to other TMDC materials and even van der Waals heterostructures. |
format |
article |
author |
Devendra Pareek Kathryna G. Roach Marco A. Gonzalez Lukas Büsing Jürgen Parisi Levent Gütay Sascha Schäfer |
author_facet |
Devendra Pareek Kathryna G. Roach Marco A. Gonzalez Lukas Büsing Jürgen Parisi Levent Gütay Sascha Schäfer |
author_sort |
Devendra Pareek |
title |
Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach |
title_short |
Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach |
title_full |
Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach |
title_fullStr |
Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach |
title_full_unstemmed |
Micro-patterned deposition of MoS2 ultrathin-films by a controlled droplet dragging approach |
title_sort |
micro-patterned deposition of mos2 ultrathin-films by a controlled droplet dragging approach |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/28e53fea417c464a92ac02e44ad933d8 |
work_keys_str_mv |
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