A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance
The morphology of zeolites influences their catalytic activity, but defining descriptors to link morphology and activity is challenging. Here, time-resolved in situ FT-IR spectroscopy and MD simulations reveal that the difference in the catalytic performance of a series of H-ZSM-5 zeolites with simi...
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Nature Portfolio
2021
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oai:doaj.org-article:29dc1529b009456782c2d3bf31c529732021-12-02T15:32:56ZA diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance10.1038/s42004-021-00543-w2399-3669https://doaj.org/article/29dc1529b009456782c2d3bf31c529732021-07-01T00:00:00Zhttps://doi.org/10.1038/s42004-021-00543-whttps://doaj.org/toc/2399-3669The morphology of zeolites influences their catalytic activity, but defining descriptors to link morphology and activity is challenging. Here, time-resolved in situ FT-IR spectroscopy and MD simulations reveal that the difference in the catalytic performance of a series of H-ZSM-5 zeolites with similar sheet-like morphology can be attributed to intracrystalline diffusive propensities in different channels.Xiaoliang LiuJing ShiGuang YangJian ZhouChuanming WangJiawei TengYangdong WangZaiku XieNature PortfolioarticleChemistryQD1-999ENCommunications Chemistry, Vol 4, Iss 1, Pp 1-10 (2021) |
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Chemistry QD1-999 |
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Chemistry QD1-999 Xiaoliang Liu Jing Shi Guang Yang Jian Zhou Chuanming Wang Jiawei Teng Yangdong Wang Zaiku Xie A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance |
description |
The morphology of zeolites influences their catalytic activity, but defining descriptors to link morphology and activity is challenging. Here, time-resolved in situ FT-IR spectroscopy and MD simulations reveal that the difference in the catalytic performance of a series of H-ZSM-5 zeolites with similar sheet-like morphology can be attributed to intracrystalline diffusive propensities in different channels. |
format |
article |
author |
Xiaoliang Liu Jing Shi Guang Yang Jian Zhou Chuanming Wang Jiawei Teng Yangdong Wang Zaiku Xie |
author_facet |
Xiaoliang Liu Jing Shi Guang Yang Jian Zhou Chuanming Wang Jiawei Teng Yangdong Wang Zaiku Xie |
author_sort |
Xiaoliang Liu |
title |
A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance |
title_short |
A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance |
title_full |
A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance |
title_fullStr |
A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance |
title_full_unstemmed |
A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance |
title_sort |
diffusion anisotropy descriptor links morphology effects of h-zsm-5 zeolites to their catalytic cracking performance |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/29dc1529b009456782c2d3bf31c52973 |
work_keys_str_mv |
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