A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance

The morphology of zeolites influences their catalytic activity, but defining descriptors to link morphology and activity is challenging. Here, time-resolved in situ FT-IR spectroscopy and MD simulations reveal that the difference in the catalytic performance of a series of H-ZSM-5 zeolites with simi...

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Autores principales: Xiaoliang Liu, Jing Shi, Guang Yang, Jian Zhou, Chuanming Wang, Jiawei Teng, Yangdong Wang, Zaiku Xie
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/29dc1529b009456782c2d3bf31c52973
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spelling oai:doaj.org-article:29dc1529b009456782c2d3bf31c529732021-12-02T15:32:56ZA diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance10.1038/s42004-021-00543-w2399-3669https://doaj.org/article/29dc1529b009456782c2d3bf31c529732021-07-01T00:00:00Zhttps://doi.org/10.1038/s42004-021-00543-whttps://doaj.org/toc/2399-3669The morphology of zeolites influences their catalytic activity, but defining descriptors to link morphology and activity is challenging. Here, time-resolved in situ FT-IR spectroscopy and MD simulations reveal that the difference in the catalytic performance of a series of H-ZSM-5 zeolites with similar sheet-like morphology can be attributed to intracrystalline diffusive propensities in different channels.Xiaoliang LiuJing ShiGuang YangJian ZhouChuanming WangJiawei TengYangdong WangZaiku XieNature PortfolioarticleChemistryQD1-999ENCommunications Chemistry, Vol 4, Iss 1, Pp 1-10 (2021)
institution DOAJ
collection DOAJ
language EN
topic Chemistry
QD1-999
spellingShingle Chemistry
QD1-999
Xiaoliang Liu
Jing Shi
Guang Yang
Jian Zhou
Chuanming Wang
Jiawei Teng
Yangdong Wang
Zaiku Xie
A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance
description The morphology of zeolites influences their catalytic activity, but defining descriptors to link morphology and activity is challenging. Here, time-resolved in situ FT-IR spectroscopy and MD simulations reveal that the difference in the catalytic performance of a series of H-ZSM-5 zeolites with similar sheet-like morphology can be attributed to intracrystalline diffusive propensities in different channels.
format article
author Xiaoliang Liu
Jing Shi
Guang Yang
Jian Zhou
Chuanming Wang
Jiawei Teng
Yangdong Wang
Zaiku Xie
author_facet Xiaoliang Liu
Jing Shi
Guang Yang
Jian Zhou
Chuanming Wang
Jiawei Teng
Yangdong Wang
Zaiku Xie
author_sort Xiaoliang Liu
title A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance
title_short A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance
title_full A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance
title_fullStr A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance
title_full_unstemmed A diffusion anisotropy descriptor links morphology effects of H-ZSM-5 zeolites to their catalytic cracking performance
title_sort diffusion anisotropy descriptor links morphology effects of h-zsm-5 zeolites to their catalytic cracking performance
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/29dc1529b009456782c2d3bf31c52973
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