Dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites

The performance of wide-bandgap perovskite photovoltaics is limited by the undesired phase transition and high density of deep level traps. Here, Tan et al. incorporate dipolar methylammonium cation to make the material defect-tolerant and achieve a high power conversion efficiency of 20.7%.

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Autores principales: Hairen Tan, Fanglin Che, Mingyang Wei, Yicheng Zhao, Makhsud I. Saidaminov, Petar Todorović, Danny Broberg, Grant Walters, Furui Tan, Taotao Zhuang, Bin Sun, Zhiqin Liang, Haifeng Yuan, Eduard Fron, Junghwan Kim, Zhenyu Yang, Oleksandr Voznyy, Mark Asta, Edward H. Sargent
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Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/29f61d7fb4174a9baf55ca8b52afb752
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spelling oai:doaj.org-article:29f61d7fb4174a9baf55ca8b52afb7522021-12-02T15:34:44ZDipolar cations confer defect tolerance in wide-bandgap metal halide perovskites10.1038/s41467-018-05531-82041-1723https://doaj.org/article/29f61d7fb4174a9baf55ca8b52afb7522018-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-05531-8https://doaj.org/toc/2041-1723The performance of wide-bandgap perovskite photovoltaics is limited by the undesired phase transition and high density of deep level traps. Here, Tan et al. incorporate dipolar methylammonium cation to make the material defect-tolerant and achieve a high power conversion efficiency of 20.7%.Hairen TanFanglin CheMingyang WeiYicheng ZhaoMakhsud I. SaidaminovPetar TodorovićDanny BrobergGrant WaltersFurui TanTaotao ZhuangBin SunZhiqin LiangHaifeng YuanEduard FronJunghwan KimZhenyu YangOleksandr VoznyyMark AstaEdward H. SargentNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-10 (2018)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Hairen Tan
Fanglin Che
Mingyang Wei
Yicheng Zhao
Makhsud I. Saidaminov
Petar Todorović
Danny Broberg
Grant Walters
Furui Tan
Taotao Zhuang
Bin Sun
Zhiqin Liang
Haifeng Yuan
Eduard Fron
Junghwan Kim
Zhenyu Yang
Oleksandr Voznyy
Mark Asta
Edward H. Sargent
Dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites
description The performance of wide-bandgap perovskite photovoltaics is limited by the undesired phase transition and high density of deep level traps. Here, Tan et al. incorporate dipolar methylammonium cation to make the material defect-tolerant and achieve a high power conversion efficiency of 20.7%.
format article
author Hairen Tan
Fanglin Che
Mingyang Wei
Yicheng Zhao
Makhsud I. Saidaminov
Petar Todorović
Danny Broberg
Grant Walters
Furui Tan
Taotao Zhuang
Bin Sun
Zhiqin Liang
Haifeng Yuan
Eduard Fron
Junghwan Kim
Zhenyu Yang
Oleksandr Voznyy
Mark Asta
Edward H. Sargent
author_facet Hairen Tan
Fanglin Che
Mingyang Wei
Yicheng Zhao
Makhsud I. Saidaminov
Petar Todorović
Danny Broberg
Grant Walters
Furui Tan
Taotao Zhuang
Bin Sun
Zhiqin Liang
Haifeng Yuan
Eduard Fron
Junghwan Kim
Zhenyu Yang
Oleksandr Voznyy
Mark Asta
Edward H. Sargent
author_sort Hairen Tan
title Dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites
title_short Dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites
title_full Dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites
title_fullStr Dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites
title_full_unstemmed Dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites
title_sort dipolar cations confer defect tolerance in wide-bandgap metal halide perovskites
publisher Nature Portfolio
publishDate 2018
url https://doaj.org/article/29f61d7fb4174a9baf55ca8b52afb752
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