Liquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality

Smart hydrogel actuators with programmable anisotropic structures present fascinating prospects considering their distinctive shape transformation and controllable environmental responsiveness under external stimuli. However, the design of anisotropic hydrogels with simple and universal fabrication...

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Autores principales: Pengli Dong, Weizhong Xu, Zhongwen Kuang, Youxing Yao, Zhiqin Zhang, Daoyou Guo, Huaping Wu, Tingyu Zhao, Aiping Liu
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Publicado: Wiley 2021
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Acceso en línea:https://doaj.org/article/2c50d1775a7041fcb8f80272ce7e40d7
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spelling oai:doaj.org-article:2c50d1775a7041fcb8f80272ce7e40d72021-11-23T07:58:49ZLiquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality2640-456710.1002/aisy.202100030https://doaj.org/article/2c50d1775a7041fcb8f80272ce7e40d72021-11-01T00:00:00Zhttps://doi.org/10.1002/aisy.202100030https://doaj.org/toc/2640-4567Smart hydrogel actuators with programmable anisotropic structures present fascinating prospects considering their distinctive shape transformation and controllable environmental responsiveness under external stimuli. However, the design of anisotropic hydrogels with simple and universal fabrication and programmable functionality is challenging for their valuable applications in smart actuators and soft robots. Herein, a simple, green, and devisable strategy is proposed to construct a heterogeneous porous hydrogel system by the different liquid diffusion (such as amyl alcohol, water, and ethanol) into a monomeric precursor solution of thermosensitive hydrogels. The well‐defined micro/nanoporous gradient and patterned structures related to selective liquid stratification and interfacial diffusion favor the fast response and accurate programmable deformation of hydrogels under temperature stimuli. Inspiringly, this simple diffusion‐driven tactic can be perfectly applicable for different responsive hydrogels with programmable multifunctionality by adding functional nanomaterials into the diffusible liquid. This green, general, and facile diffusion‐driven strategy provides significant guidance for fabricating environmentally responsive hydrogels with tailorable functionality for their multipurpose applications in drug delivery, bioengineering, smart actuators, and soft robots.Pengli DongWeizhong XuZhongwen KuangYouxing YaoZhiqin ZhangDaoyou GuoHuaping WuTingyu ZhaoAiping LiuWileyarticleanisotropic hydrogelsinterfacial diffusionliquid stratificationprogrammable functionalitiessmart actuatorsComputer engineering. Computer hardwareTK7885-7895Control engineering systems. Automatic machinery (General)TJ212-225ENAdvanced Intelligent Systems, Vol 3, Iss 11, Pp n/a-n/a (2021)
institution DOAJ
collection DOAJ
language EN
topic anisotropic hydrogels
interfacial diffusion
liquid stratification
programmable functionalities
smart actuators
Computer engineering. Computer hardware
TK7885-7895
Control engineering systems. Automatic machinery (General)
TJ212-225
spellingShingle anisotropic hydrogels
interfacial diffusion
liquid stratification
programmable functionalities
smart actuators
Computer engineering. Computer hardware
TK7885-7895
Control engineering systems. Automatic machinery (General)
TJ212-225
Pengli Dong
Weizhong Xu
Zhongwen Kuang
Youxing Yao
Zhiqin Zhang
Daoyou Guo
Huaping Wu
Tingyu Zhao
Aiping Liu
Liquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality
description Smart hydrogel actuators with programmable anisotropic structures present fascinating prospects considering their distinctive shape transformation and controllable environmental responsiveness under external stimuli. However, the design of anisotropic hydrogels with simple and universal fabrication and programmable functionality is challenging for their valuable applications in smart actuators and soft robots. Herein, a simple, green, and devisable strategy is proposed to construct a heterogeneous porous hydrogel system by the different liquid diffusion (such as amyl alcohol, water, and ethanol) into a monomeric precursor solution of thermosensitive hydrogels. The well‐defined micro/nanoporous gradient and patterned structures related to selective liquid stratification and interfacial diffusion favor the fast response and accurate programmable deformation of hydrogels under temperature stimuli. Inspiringly, this simple diffusion‐driven tactic can be perfectly applicable for different responsive hydrogels with programmable multifunctionality by adding functional nanomaterials into the diffusible liquid. This green, general, and facile diffusion‐driven strategy provides significant guidance for fabricating environmentally responsive hydrogels with tailorable functionality for their multipurpose applications in drug delivery, bioengineering, smart actuators, and soft robots.
format article
author Pengli Dong
Weizhong Xu
Zhongwen Kuang
Youxing Yao
Zhiqin Zhang
Daoyou Guo
Huaping Wu
Tingyu Zhao
Aiping Liu
author_facet Pengli Dong
Weizhong Xu
Zhongwen Kuang
Youxing Yao
Zhiqin Zhang
Daoyou Guo
Huaping Wu
Tingyu Zhao
Aiping Liu
author_sort Pengli Dong
title Liquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality
title_short Liquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality
title_full Liquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality
title_fullStr Liquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality
title_full_unstemmed Liquid Stratification and Diffusion‐Induced Anisotropic Hydrogel Actuators with Excellent Thermosensitivity and Programmable Functionality
title_sort liquid stratification and diffusion‐induced anisotropic hydrogel actuators with excellent thermosensitivity and programmable functionality
publisher Wiley
publishDate 2021
url https://doaj.org/article/2c50d1775a7041fcb8f80272ce7e40d7
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