Enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer

In this work, strontium titanate (STO) was coated on the surface of carbon nanotubes (MWCNTs) through a sol–gel method to form a core–shell structure hybrid powder (STO@MWCNTs). This powder was then added to polydimethylsiloxane to prepare a flexible high-K composite. As coating, STO effectively pre...

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Autores principales: Han Ruolin, Liu Yuping, Shi Jinchao, Chen Guang-Xin, Li Qifang
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Lenguaje:EN
Publicado: De Gruyter 2021
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Acceso en línea:https://doaj.org/article/2d5f0827c64d4c919d91c8d375235e39
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spelling oai:doaj.org-article:2d5f0827c64d4c919d91c8d375235e392021-12-05T14:10:47ZEnhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer1618-722910.1515/epoly-2021-0028https://doaj.org/article/2d5f0827c64d4c919d91c8d375235e392021-04-01T00:00:00Zhttps://doi.org/10.1515/epoly-2021-0028https://doaj.org/toc/1618-7229In this work, strontium titanate (STO) was coated on the surface of carbon nanotubes (MWCNTs) through a sol–gel method to form a core–shell structure hybrid powder (STO@MWCNTs). This powder was then added to polydimethylsiloxane to prepare a flexible high-K composite. As coating, STO effectively prevents the overlap and agglomeration of MWCNTs, thereby passivating the percolation threshold of the composite. STO increases the dielectric properties of the composite as a high dielectric ceramic. Under a low filler loading amount of 11 wt%, the dielectric constant and dielectric loss of the composite are 53 and 0.1, respectively. In addition, the composite can still maintain superior breakdown strength and mechanical properties, given the relatively low filler concentration. The enhanced dielectric properties, breakdown strength, and tensile strength make the composite suitable for application as dielectric material in flexible and stretchable energy storage equipment.Han RuolinLiu YupingShi JinchaoChen Guang-XinLi QifangDe Gruyterarticlecarbon nanotubesstrontium titanatesol–gel methodcompositesPolymers and polymer manufactureTP1080-1185ENe-Polymers, Vol 21, Iss 1, Pp 272-278 (2021)
institution DOAJ
collection DOAJ
language EN
topic carbon nanotubes
strontium titanate
sol–gel method
composites
Polymers and polymer manufacture
TP1080-1185
spellingShingle carbon nanotubes
strontium titanate
sol–gel method
composites
Polymers and polymer manufacture
TP1080-1185
Han Ruolin
Liu Yuping
Shi Jinchao
Chen Guang-Xin
Li Qifang
Enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer
description In this work, strontium titanate (STO) was coated on the surface of carbon nanotubes (MWCNTs) through a sol–gel method to form a core–shell structure hybrid powder (STO@MWCNTs). This powder was then added to polydimethylsiloxane to prepare a flexible high-K composite. As coating, STO effectively prevents the overlap and agglomeration of MWCNTs, thereby passivating the percolation threshold of the composite. STO increases the dielectric properties of the composite as a high dielectric ceramic. Under a low filler loading amount of 11 wt%, the dielectric constant and dielectric loss of the composite are 53 and 0.1, respectively. In addition, the composite can still maintain superior breakdown strength and mechanical properties, given the relatively low filler concentration. The enhanced dielectric properties, breakdown strength, and tensile strength make the composite suitable for application as dielectric material in flexible and stretchable energy storage equipment.
format article
author Han Ruolin
Liu Yuping
Shi Jinchao
Chen Guang-Xin
Li Qifang
author_facet Han Ruolin
Liu Yuping
Shi Jinchao
Chen Guang-Xin
Li Qifang
author_sort Han Ruolin
title Enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer
title_short Enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer
title_full Enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer
title_fullStr Enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer
title_full_unstemmed Enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an SrTiO3 layer
title_sort enhanced dielectric properties and breakdown strength of polymer/carbon nanotube composites by coating an srtio3 layer
publisher De Gruyter
publishDate 2021
url https://doaj.org/article/2d5f0827c64d4c919d91c8d375235e39
work_keys_str_mv AT hanruolin enhanceddielectricpropertiesandbreakdownstrengthofpolymercarbonnanotubecompositesbycoatingansrtio3layer
AT liuyuping enhanceddielectricpropertiesandbreakdownstrengthofpolymercarbonnanotubecompositesbycoatingansrtio3layer
AT shijinchao enhanceddielectricpropertiesandbreakdownstrengthofpolymercarbonnanotubecompositesbycoatingansrtio3layer
AT chenguangxin enhanceddielectricpropertiesandbreakdownstrengthofpolymercarbonnanotubecompositesbycoatingansrtio3layer
AT liqifang enhanceddielectricpropertiesandbreakdownstrengthofpolymercarbonnanotubecompositesbycoatingansrtio3layer
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