Titanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss

Abstract Realising engineering ceramics to serve as substrate materials in high-performance terahertz(THz) that are low-cost, have low dielectric loss and near-dispersionless broadband, high permittivity, is exceedingly demanding. Such substrates are deployed in, for example, integrated circuits for...

Descripción completa

Guardado en:
Detalles Bibliográficos
Autores principales: Chuying Yu, Yang Zeng, Bin Yang, Robert Donnan, Jinbao Huang, Zhaoxian Xiong, Amit Mahajan, Baogui Shi, Haitao Ye, Russell Binions, Nadezda V. Tarakina, Mike J Reece, Haixue Yan
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2017
Materias:
R
Q
Acceso en línea:https://doaj.org/article/30d2c227327145c6b3f495db60d4a5b3
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
id oai:doaj.org-article:30d2c227327145c6b3f495db60d4a5b3
record_format dspace
spelling oai:doaj.org-article:30d2c227327145c6b3f495db60d4a5b32021-12-02T16:06:27ZTitanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss10.1038/s41598-017-07019-92045-2322https://doaj.org/article/30d2c227327145c6b3f495db60d4a5b32017-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-07019-9https://doaj.org/toc/2045-2322Abstract Realising engineering ceramics to serve as substrate materials in high-performance terahertz(THz) that are low-cost, have low dielectric loss and near-dispersionless broadband, high permittivity, is exceedingly demanding. Such substrates are deployed in, for example, integrated circuits for synthesizing and converting nonplanar and 3D structures into planar forms. The Rutile form of titanium dioxide (TiO2) has been widely accepted as commercially economical candidate substrate that meets demands for both low-loss and high permittivities at sub-THz bands. However, the relationship between its mechanisms of dielectric response to the microstructure have never been systematically investigated in order to engineer ultra-low dielectric-loss and high value, dispersionless permittivities. Here we show TiO2 THz dielectrics with high permittivity (ca. 102.30) and ultra-low loss (ca. 0.0042). These were prepared by insight gleaned from a broad use of materials characterisation methods to successfully engineer porosities, second phase, crystallography shear-planes and oxygen vacancies during sintering. The dielectric loss achieved here is not only with negligible dispersion over 0.2–0.8 THz, but also has the lowest value measured for known high-permittivity dielectrics. We expect the insight afforded by this study will underpin the development of subwavelength-scale, planar integrated circuits, compact high Q-resonators and broadband, slow-light devices in the THz band.Chuying YuYang ZengBin YangRobert DonnanJinbao HuangZhaoxian XiongAmit MahajanBaogui ShiHaitao YeRussell BinionsNadezda V. TarakinaMike J ReeceHaixue YanNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-9 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Chuying Yu
Yang Zeng
Bin Yang
Robert Donnan
Jinbao Huang
Zhaoxian Xiong
Amit Mahajan
Baogui Shi
Haitao Ye
Russell Binions
Nadezda V. Tarakina
Mike J Reece
Haixue Yan
Titanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss
description Abstract Realising engineering ceramics to serve as substrate materials in high-performance terahertz(THz) that are low-cost, have low dielectric loss and near-dispersionless broadband, high permittivity, is exceedingly demanding. Such substrates are deployed in, for example, integrated circuits for synthesizing and converting nonplanar and 3D structures into planar forms. The Rutile form of titanium dioxide (TiO2) has been widely accepted as commercially economical candidate substrate that meets demands for both low-loss and high permittivities at sub-THz bands. However, the relationship between its mechanisms of dielectric response to the microstructure have never been systematically investigated in order to engineer ultra-low dielectric-loss and high value, dispersionless permittivities. Here we show TiO2 THz dielectrics with high permittivity (ca. 102.30) and ultra-low loss (ca. 0.0042). These were prepared by insight gleaned from a broad use of materials characterisation methods to successfully engineer porosities, second phase, crystallography shear-planes and oxygen vacancies during sintering. The dielectric loss achieved here is not only with negligible dispersion over 0.2–0.8 THz, but also has the lowest value measured for known high-permittivity dielectrics. We expect the insight afforded by this study will underpin the development of subwavelength-scale, planar integrated circuits, compact high Q-resonators and broadband, slow-light devices in the THz band.
format article
author Chuying Yu
Yang Zeng
Bin Yang
Robert Donnan
Jinbao Huang
Zhaoxian Xiong
Amit Mahajan
Baogui Shi
Haitao Ye
Russell Binions
Nadezda V. Tarakina
Mike J Reece
Haixue Yan
author_facet Chuying Yu
Yang Zeng
Bin Yang
Robert Donnan
Jinbao Huang
Zhaoxian Xiong
Amit Mahajan
Baogui Shi
Haitao Ye
Russell Binions
Nadezda V. Tarakina
Mike J Reece
Haixue Yan
author_sort Chuying Yu
title Titanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss
title_short Titanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss
title_full Titanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss
title_fullStr Titanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss
title_full_unstemmed Titanium Dioxide Engineered for Near-dispersionless High Terahertz Permittivity and Ultra-low-loss
title_sort titanium dioxide engineered for near-dispersionless high terahertz permittivity and ultra-low-loss
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/30d2c227327145c6b3f495db60d4a5b3
work_keys_str_mv AT chuyingyu titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT yangzeng titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT binyang titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT robertdonnan titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT jinbaohuang titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT zhaoxianxiong titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT amitmahajan titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT baoguishi titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT haitaoye titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT russellbinions titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT nadezdavtarakina titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT mikejreece titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
AT haixueyan titaniumdioxideengineeredforneardispersionlesshighterahertzpermittivityandultralowloss
_version_ 1718384953386860544