Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal
Understanding the solid–electrolyte interphase (SEI) is key to developing safe dendrite-free lithium batteries. Here, by exploiting the electrons in lithium metal to selectively hyperpolarise the NMR signals, the authors reveal the chemistry and spatial distribution of species at the metal–SEI inter...
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Nature Portfolio
2020
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oai:doaj.org-article:31ed0fe03eb04b7bb53620250b25a05f2021-12-02T16:49:44ZSelective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal10.1038/s41467-020-16114-x2041-1723https://doaj.org/article/31ed0fe03eb04b7bb53620250b25a05f2020-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-16114-xhttps://doaj.org/toc/2041-1723Understanding the solid–electrolyte interphase (SEI) is key to developing safe dendrite-free lithium batteries. Here, by exploiting the electrons in lithium metal to selectively hyperpolarise the NMR signals, the authors reveal the chemistry and spatial distribution of species at the metal–SEI interface.Michael A. HopeBernardine L. D. RinkelAnna B. GunnarsdóttirKatharina MärkerSvetlana MenkinSubhradip PaulIvan V. SergeyevClare P. GreyNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-8 (2020) |
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Science Q Michael A. Hope Bernardine L. D. Rinkel Anna B. Gunnarsdóttir Katharina Märker Svetlana Menkin Subhradip Paul Ivan V. Sergeyev Clare P. Grey Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal |
description |
Understanding the solid–electrolyte interphase (SEI) is key to developing safe dendrite-free lithium batteries. Here, by exploiting the electrons in lithium metal to selectively hyperpolarise the NMR signals, the authors reveal the chemistry and spatial distribution of species at the metal–SEI interface. |
format |
article |
author |
Michael A. Hope Bernardine L. D. Rinkel Anna B. Gunnarsdóttir Katharina Märker Svetlana Menkin Subhradip Paul Ivan V. Sergeyev Clare P. Grey |
author_facet |
Michael A. Hope Bernardine L. D. Rinkel Anna B. Gunnarsdóttir Katharina Märker Svetlana Menkin Subhradip Paul Ivan V. Sergeyev Clare P. Grey |
author_sort |
Michael A. Hope |
title |
Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal |
title_short |
Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal |
title_full |
Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal |
title_fullStr |
Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal |
title_full_unstemmed |
Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal |
title_sort |
selective nmr observation of the sei–metal interface by dynamic nuclear polarisation from lithium metal |
publisher |
Nature Portfolio |
publishDate |
2020 |
url |
https://doaj.org/article/31ed0fe03eb04b7bb53620250b25a05f |
work_keys_str_mv |
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1718383206721388544 |