Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal

Understanding the solid–electrolyte interphase (SEI) is key to developing safe dendrite-free lithium batteries. Here, by exploiting the electrons in lithium metal to selectively hyperpolarise the NMR signals, the authors reveal the chemistry and spatial distribution of species at the metal–SEI inter...

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Autores principales: Michael A. Hope, Bernardine L. D. Rinkel, Anna B. Gunnarsdóttir, Katharina Märker, Svetlana Menkin, Subhradip Paul, Ivan V. Sergeyev, Clare P. Grey
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Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/31ed0fe03eb04b7bb53620250b25a05f
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spelling oai:doaj.org-article:31ed0fe03eb04b7bb53620250b25a05f2021-12-02T16:49:44ZSelective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal10.1038/s41467-020-16114-x2041-1723https://doaj.org/article/31ed0fe03eb04b7bb53620250b25a05f2020-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-16114-xhttps://doaj.org/toc/2041-1723Understanding the solid–electrolyte interphase (SEI) is key to developing safe dendrite-free lithium batteries. Here, by exploiting the electrons in lithium metal to selectively hyperpolarise the NMR signals, the authors reveal the chemistry and spatial distribution of species at the metal–SEI interface.Michael A. HopeBernardine L. D. RinkelAnna B. GunnarsdóttirKatharina MärkerSvetlana MenkinSubhradip PaulIvan V. SergeyevClare P. GreyNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-8 (2020)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Michael A. Hope
Bernardine L. D. Rinkel
Anna B. Gunnarsdóttir
Katharina Märker
Svetlana Menkin
Subhradip Paul
Ivan V. Sergeyev
Clare P. Grey
Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal
description Understanding the solid–electrolyte interphase (SEI) is key to developing safe dendrite-free lithium batteries. Here, by exploiting the electrons in lithium metal to selectively hyperpolarise the NMR signals, the authors reveal the chemistry and spatial distribution of species at the metal–SEI interface.
format article
author Michael A. Hope
Bernardine L. D. Rinkel
Anna B. Gunnarsdóttir
Katharina Märker
Svetlana Menkin
Subhradip Paul
Ivan V. Sergeyev
Clare P. Grey
author_facet Michael A. Hope
Bernardine L. D. Rinkel
Anna B. Gunnarsdóttir
Katharina Märker
Svetlana Menkin
Subhradip Paul
Ivan V. Sergeyev
Clare P. Grey
author_sort Michael A. Hope
title Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal
title_short Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal
title_full Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal
title_fullStr Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal
title_full_unstemmed Selective NMR observation of the SEI–metal interface by dynamic nuclear polarisation from lithium metal
title_sort selective nmr observation of the sei–metal interface by dynamic nuclear polarisation from lithium metal
publisher Nature Portfolio
publishDate 2020
url https://doaj.org/article/31ed0fe03eb04b7bb53620250b25a05f
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