Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2

Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2

The photocatalytic conversion of CH4 into CH3OH with high activity and selectivity must avoid product overoxidation. Here, authors minimize overoxidation by using a (001)-dominated TiO2 nanosheet to circumvent CH4 overoxidation intermediates plus reaction pathways that occur on (101) facets.

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Autores principales: Ningdong Feng, Huiwen Lin, Hui Song, Longxiao Yang, Daiming Tang, Feng Deng, Jinhua Ye
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/328f05efbf6c44b2a230ce9aeb0ffe42
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spelling oai:doaj.org-article:328f05efbf6c44b2a230ce9aeb0ffe422021-12-02T18:49:35ZEfficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO210.1038/s41467-021-24912-02041-1723https://doaj.org/article/328f05efbf6c44b2a230ce9aeb0ffe422021-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-24912-0https://doaj.org/toc/2041-1723The photocatalytic conversion of CH4 into CH3OH with high activity and selectivity must avoid product overoxidation. Here, authors minimize overoxidation by using a (001)-dominated TiO2 nanosheet to circumvent CH4 overoxidation intermediates plus reaction pathways that occur on (101) facets.Ningdong FengHuiwen LinHui SongLongxiao YangDaiming TangFeng DengJinhua YeNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-10 (2021)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Ningdong Feng
Huiwen Lin
Hui Song
Longxiao Yang
Daiming Tang
Feng Deng
Jinhua Ye
Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2
description The photocatalytic conversion of CH4 into CH3OH with high activity and selectivity must avoid product overoxidation. Here, authors minimize overoxidation by using a (001)-dominated TiO2 nanosheet to circumvent CH4 overoxidation intermediates plus reaction pathways that occur on (101) facets.
format article
author Ningdong Feng
Huiwen Lin
Hui Song
Longxiao Yang
Daiming Tang
Feng Deng
Jinhua Ye
author_facet Ningdong Feng
Huiwen Lin
Hui Song
Longxiao Yang
Daiming Tang
Feng Deng
Jinhua Ye
author_sort Ningdong Feng
title Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2
title_short Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2
title_full Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2
title_fullStr Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2
title_full_unstemmed Efficient and selective photocatalytic CH4 conversion to CH3OH with O2 by controlling overoxidation on TiO2
title_sort efficient and selective photocatalytic ch4 conversion to ch3oh with o2 by controlling overoxidation on tio2
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/328f05efbf6c44b2a230ce9aeb0ffe42
work_keys_str_mv AT ningdongfeng efficientandselectivephotocatalyticch4conversiontoch3ohwitho2bycontrollingoveroxidationontio2
AT huiwenlin efficientandselectivephotocatalyticch4conversiontoch3ohwitho2bycontrollingoveroxidationontio2
AT huisong efficientandselectivephotocatalyticch4conversiontoch3ohwitho2bycontrollingoveroxidationontio2
AT longxiaoyang efficientandselectivephotocatalyticch4conversiontoch3ohwitho2bycontrollingoveroxidationontio2
AT daimingtang efficientandselectivephotocatalyticch4conversiontoch3ohwitho2bycontrollingoveroxidationontio2
AT fengdeng efficientandselectivephotocatalyticch4conversiontoch3ohwitho2bycontrollingoveroxidationontio2
AT jinhuaye efficientandselectivephotocatalyticch4conversiontoch3ohwitho2bycontrollingoveroxidationontio2
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