Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation

Covalent organic frameworks are potential catalysts for nitrogen reduction, but limited nitrogen transport restricts the utilization ratio of active sites. Here, the authors demonstrate that electrochemical excitation of covalent organic frameworks can lead to efficient nitrogen reduction.

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Autores principales:	Sisi Liu, Mengfan Wang, Tao Qian, Haoqing Ji, Jie Liu, Chenglin Yan
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2019
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/329a6ccd62704c6a8c93d06d40f89d82
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spelling	oai:doaj.org-article:329a6ccd62704c6a8c93d06d40f89d822021-12-02T15:35:09ZFacilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation10.1038/s41467-019-11846-x2041-1723https://doaj.org/article/329a6ccd62704c6a8c93d06d40f89d822019-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-11846-xhttps://doaj.org/toc/2041-1723Covalent organic frameworks are potential catalysts for nitrogen reduction, but limited nitrogen transport restricts the utilization ratio of active sites. Here, the authors demonstrate that electrochemical excitation of covalent organic frameworks can lead to efficient nitrogen reduction.Sisi LiuMengfan WangTao QianHaoqing JiJie LiuChenglin YanNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-9 (2019)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Sisi Liu Mengfan Wang Tao Qian Haoqing Ji Jie Liu Chenglin Yan Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation
description	Covalent organic frameworks are potential catalysts for nitrogen reduction, but limited nitrogen transport restricts the utilization ratio of active sites. Here, the authors demonstrate that electrochemical excitation of covalent organic frameworks can lead to efficient nitrogen reduction.
format	article
author	Sisi Liu Mengfan Wang Tao Qian Haoqing Ji Jie Liu Chenglin Yan
author_facet	Sisi Liu Mengfan Wang Tao Qian Haoqing Ji Jie Liu Chenglin Yan
author_sort	Sisi Liu
title	Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation
title_short	Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation
title_full	Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation
title_fullStr	Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation
title_full_unstemmed	Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation
title_sort	facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation
publisher	Nature Portfolio
publishDate	2019
url	https://doaj.org/article/329a6ccd62704c6a8c93d06d40f89d82
work_keys_str_mv	AT sisiliu facilitatingnitrogenaccessibilitytoboronrichcovalentorganicframeworksviaelectrochemicalexcitationforefficientnitrogenfixation AT mengfanwang facilitatingnitrogenaccessibilitytoboronrichcovalentorganicframeworksviaelectrochemicalexcitationforefficientnitrogenfixation AT taoqian facilitatingnitrogenaccessibilitytoboronrichcovalentorganicframeworksviaelectrochemicalexcitationforefficientnitrogenfixation AT haoqingji facilitatingnitrogenaccessibilitytoboronrichcovalentorganicframeworksviaelectrochemicalexcitationforefficientnitrogenfixation AT jieliu facilitatingnitrogenaccessibilitytoboronrichcovalentorganicframeworksviaelectrochemicalexcitationforefficientnitrogenfixation AT chenglinyan facilitatingnitrogenaccessibilitytoboronrichcovalentorganicframeworksviaelectrochemicalexcitationforefficientnitrogenfixation
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Facilitating nitrogen accessibility to boron-rich covalent organic frameworks via electrochemical excitation for efficient nitrogen fixation

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