Ultrafast coherence transfer in DNA-templated silver nanoclusters
DNA-templated silver nanoclusters possess desirable optical properties, but their excited state dynamics remain poorly understood. Here the authors show that intracluster relaxations in such clusters are strongly coupled to a vibrational mode, resulting in ultrafast concerted transfer of population...
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Nature Portfolio
2017
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oai:doaj.org-article:354f508e23fc4b85834f84712f9fe92d2021-12-02T14:40:33ZUltrafast coherence transfer in DNA-templated silver nanoclusters10.1038/ncomms155772041-1723https://doaj.org/article/354f508e23fc4b85834f84712f9fe92d2017-05-01T00:00:00Zhttps://doi.org/10.1038/ncomms15577https://doaj.org/toc/2041-1723DNA-templated silver nanoclusters possess desirable optical properties, but their excited state dynamics remain poorly understood. Here the authors show that intracluster relaxations in such clusters are strongly coupled to a vibrational mode, resulting in ultrafast concerted transfer of population and coherence between excited states.Erling ThyrhaugSidsel Ammitzbøll BoghMiguel R Carro-TembouryCharlotte Stahl MadsenTom VoschDonatas ZigmantasNature PortfolioarticleScienceQENNature Communications, Vol 8, Iss 1, Pp 1-7 (2017) |
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Science Q Erling Thyrhaug Sidsel Ammitzbøll Bogh Miguel R Carro-Temboury Charlotte Stahl Madsen Tom Vosch Donatas Zigmantas Ultrafast coherence transfer in DNA-templated silver nanoclusters |
description |
DNA-templated silver nanoclusters possess desirable optical properties, but their excited state dynamics remain poorly understood. Here the authors show that intracluster relaxations in such clusters are strongly coupled to a vibrational mode, resulting in ultrafast concerted transfer of population and coherence between excited states. |
format |
article |
author |
Erling Thyrhaug Sidsel Ammitzbøll Bogh Miguel R Carro-Temboury Charlotte Stahl Madsen Tom Vosch Donatas Zigmantas |
author_facet |
Erling Thyrhaug Sidsel Ammitzbøll Bogh Miguel R Carro-Temboury Charlotte Stahl Madsen Tom Vosch Donatas Zigmantas |
author_sort |
Erling Thyrhaug |
title |
Ultrafast coherence transfer in DNA-templated silver nanoclusters |
title_short |
Ultrafast coherence transfer in DNA-templated silver nanoclusters |
title_full |
Ultrafast coherence transfer in DNA-templated silver nanoclusters |
title_fullStr |
Ultrafast coherence transfer in DNA-templated silver nanoclusters |
title_full_unstemmed |
Ultrafast coherence transfer in DNA-templated silver nanoclusters |
title_sort |
ultrafast coherence transfer in dna-templated silver nanoclusters |
publisher |
Nature Portfolio |
publishDate |
2017 |
url |
https://doaj.org/article/354f508e23fc4b85834f84712f9fe92d |
work_keys_str_mv |
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_version_ |
1718390229325316096 |