Coherence in carotenoid-to-chlorophyll energy transfer

Energy transfer from carotenoids to chlorophylls in light-harvesting is still not fully understood, especially in the ultrafast regime. Here, the authors investigate the coherent dynamics of this process in peridinin-chlorophyll a-protein complex via 2D electronic spectroscopy and quantum chemical c...

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Autores principales: Elena Meneghin, Andrea Volpato, Lorenzo Cupellini, Luca Bolzonello, Sandro Jurinovich, Vincenzo Mascoli, Donatella Carbonera, Benedetta Mennucci, Elisabetta Collini
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2018
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Acceso en línea:https://doaj.org/article/37804a14d2fc46a1adbada56c15350fc
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Sumario:Energy transfer from carotenoids to chlorophylls in light-harvesting is still not fully understood, especially in the ultrafast regime. Here, the authors investigate the coherent dynamics of this process in peridinin-chlorophyll a-protein complex via 2D electronic spectroscopy and quantum chemical calculations.