Band Structure of Topological Insulator BiSbTe1.25Se1.75

Abstract We present our angle resolved photoelectron spectroscopy (ARPES) and density functional theory results on quaternary topological insulator (TI) BiSbTe1.25Se1.75 (BSTS) confirming the non-trivial topology of the surface state bands (SSBs) in this compound. We find that the SSBs, which are ar...

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Autores principales: H. Lohani, P. Mishra, A. Banerjee, K. Majhi, R. Ganesan, U. Manju, D. Topwal, P. S. Anil Kumar, B. R. Sekhar
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Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/38c97926060c495cafa8809f537eb78a
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spelling oai:doaj.org-article:38c97926060c495cafa8809f537eb78a2021-12-02T12:32:32ZBand Structure of Topological Insulator BiSbTe1.25Se1.7510.1038/s41598-017-04985-y2045-2322https://doaj.org/article/38c97926060c495cafa8809f537eb78a2017-07-01T00:00:00Zhttps://doi.org/10.1038/s41598-017-04985-yhttps://doaj.org/toc/2045-2322Abstract We present our angle resolved photoelectron spectroscopy (ARPES) and density functional theory results on quaternary topological insulator (TI) BiSbTe1.25Se1.75 (BSTS) confirming the non-trivial topology of the surface state bands (SSBs) in this compound. We find that the SSBs, which are are sensitive to the atomic composition of the terminating surface have a partial 3D character. Our detailed study of the band bending (BB) effects shows that in BSTS the Dirac point (DP) shifts by more than two times compared to that in Bi2Se3 to reach the saturation. The stronger BB in BSTS could be due to the difference in screening of the surface charges. From momentum density curves (MDCs) of the ARPES data we obtained an energy dispersion relation showing the warping strength of the Fermi surface in BSTS to be intermediate between those found in Bi2Se3 and Bi2Te3 and also to be tunable by controlling the ratio of chalcogen/pnictogen atoms. Our experiments also reveal that the nature of the BB effects are highly sensitive to the exposure of the fresh surface to various gas species. These findings have important implications in the tuning of DP in TIs for technological applications.H. LohaniP. MishraA. BanerjeeK. MajhiR. GanesanU. ManjuD. TopwalP. S. Anil KumarB. R. SekharNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 7, Iss 1, Pp 1-10 (2017)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
H. Lohani
P. Mishra
A. Banerjee
K. Majhi
R. Ganesan
U. Manju
D. Topwal
P. S. Anil Kumar
B. R. Sekhar
Band Structure of Topological Insulator BiSbTe1.25Se1.75
description Abstract We present our angle resolved photoelectron spectroscopy (ARPES) and density functional theory results on quaternary topological insulator (TI) BiSbTe1.25Se1.75 (BSTS) confirming the non-trivial topology of the surface state bands (SSBs) in this compound. We find that the SSBs, which are are sensitive to the atomic composition of the terminating surface have a partial 3D character. Our detailed study of the band bending (BB) effects shows that in BSTS the Dirac point (DP) shifts by more than two times compared to that in Bi2Se3 to reach the saturation. The stronger BB in BSTS could be due to the difference in screening of the surface charges. From momentum density curves (MDCs) of the ARPES data we obtained an energy dispersion relation showing the warping strength of the Fermi surface in BSTS to be intermediate between those found in Bi2Se3 and Bi2Te3 and also to be tunable by controlling the ratio of chalcogen/pnictogen atoms. Our experiments also reveal that the nature of the BB effects are highly sensitive to the exposure of the fresh surface to various gas species. These findings have important implications in the tuning of DP in TIs for technological applications.
format article
author H. Lohani
P. Mishra
A. Banerjee
K. Majhi
R. Ganesan
U. Manju
D. Topwal
P. S. Anil Kumar
B. R. Sekhar
author_facet H. Lohani
P. Mishra
A. Banerjee
K. Majhi
R. Ganesan
U. Manju
D. Topwal
P. S. Anil Kumar
B. R. Sekhar
author_sort H. Lohani
title Band Structure of Topological Insulator BiSbTe1.25Se1.75
title_short Band Structure of Topological Insulator BiSbTe1.25Se1.75
title_full Band Structure of Topological Insulator BiSbTe1.25Se1.75
title_fullStr Band Structure of Topological Insulator BiSbTe1.25Se1.75
title_full_unstemmed Band Structure of Topological Insulator BiSbTe1.25Se1.75
title_sort band structure of topological insulator bisbte1.25se1.75
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/38c97926060c495cafa8809f537eb78a
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