Effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition
Abstract In this study, silicon (Si) was doped on a tetrahedral amorphous carbon (ta-C) coating and the tribological characteristics of the resulting Si-doped diamond-like carbon (DLC; a-C:Si:H) were investigated against a SUJ2 ball. The Si fraction in the coating was varied from 0 to ~ 20 at.% by i...
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2021
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oai:doaj.org-article:39222e35881e4657a6876f62c480ad432021-12-02T14:11:31ZEffects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition10.1038/s41598-021-83158-42045-2322https://doaj.org/article/39222e35881e4657a6876f62c480ad432021-02-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-83158-4https://doaj.org/toc/2045-2322Abstract In this study, silicon (Si) was doped on a tetrahedral amorphous carbon (ta-C) coating and the tribological characteristics of the resulting Si-doped diamond-like carbon (DLC; a-C:Si:H) were investigated against a SUJ2 ball. The Si fraction in the coating was varied from 0 to ~ 20 at.% by increasing the trimethylsilane gas flow rate during filtered cathodic vacuum arc deposition. The coefficient of friction (CoF) showed no obvious change when the Si fraction was less than ~ 7 at.%. However, after Si doping, it significantly decreased when the Si fraction was greater than ~ 8 at.%. The running-in period also decreased to less than 1000 cycles after Si doping. The rapid formation of Si-rich debris and transfer layer led to the fabrication of a low-friction tribofilm, which was induced by the tribochemical reaction with moisture under ambient conditions. When the Si fraction was ~ 17 at.%, the lowest CoF of less than 0.05 was obtained. Further Si doping beyond the critical point led to the destruction of the film because of reduced hardness.Jae-Il KimYoung-Jun JangJisoo KimJongkuk KimNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-13 (2021) |
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Medicine R Science Q Jae-Il Kim Young-Jun Jang Jisoo Kim Jongkuk Kim Effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition |
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Abstract In this study, silicon (Si) was doped on a tetrahedral amorphous carbon (ta-C) coating and the tribological characteristics of the resulting Si-doped diamond-like carbon (DLC; a-C:Si:H) were investigated against a SUJ2 ball. The Si fraction in the coating was varied from 0 to ~ 20 at.% by increasing the trimethylsilane gas flow rate during filtered cathodic vacuum arc deposition. The coefficient of friction (CoF) showed no obvious change when the Si fraction was less than ~ 7 at.%. However, after Si doping, it significantly decreased when the Si fraction was greater than ~ 8 at.%. The running-in period also decreased to less than 1000 cycles after Si doping. The rapid formation of Si-rich debris and transfer layer led to the fabrication of a low-friction tribofilm, which was induced by the tribochemical reaction with moisture under ambient conditions. When the Si fraction was ~ 17 at.%, the lowest CoF of less than 0.05 was obtained. Further Si doping beyond the critical point led to the destruction of the film because of reduced hardness. |
format |
article |
author |
Jae-Il Kim Young-Jun Jang Jisoo Kim Jongkuk Kim |
author_facet |
Jae-Il Kim Young-Jun Jang Jisoo Kim Jongkuk Kim |
author_sort |
Jae-Il Kim |
title |
Effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition |
title_short |
Effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition |
title_full |
Effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition |
title_fullStr |
Effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition |
title_full_unstemmed |
Effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition |
title_sort |
effects of silicon doping on low-friction and high-hardness diamond-like carbon coating via filtered cathodic vacuum arc deposition |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/39222e35881e4657a6876f62c480ad43 |
work_keys_str_mv |
AT jaeilkim effectsofsilicondopingonlowfrictionandhighhardnessdiamondlikecarboncoatingviafilteredcathodicvacuumarcdeposition AT youngjunjang effectsofsilicondopingonlowfrictionandhighhardnessdiamondlikecarboncoatingviafilteredcathodicvacuumarcdeposition AT jisookim effectsofsilicondopingonlowfrictionandhighhardnessdiamondlikecarboncoatingviafilteredcathodicvacuumarcdeposition AT jongkukkim effectsofsilicondopingonlowfrictionandhighhardnessdiamondlikecarboncoatingviafilteredcathodicvacuumarcdeposition |
_version_ |
1718391835373600768 |