Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence

Knowing the photophysics of thermally-activated delayed fluorescence (TADF) is crucial when designing organic light emitting diodes. Here the authors show that spin orbit coupling in TADF materials is described by a second order vibronic coupling mechanism, and demonstrate the importance of resonanc...

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Autores principales:	Marc K. Etherington, Jamie Gibson, Heather F. Higginbotham, Thomas J. Penfold, Andrew P. Monkman
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2016
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/3abe5e68e1034e658db51689cca04181
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spelling	oai:doaj.org-article:3abe5e68e1034e658db51689cca041812021-12-02T17:32:22ZRevealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence10.1038/ncomms136802041-1723https://doaj.org/article/3abe5e68e1034e658db51689cca041812016-11-01T00:00:00Zhttps://doi.org/10.1038/ncomms13680https://doaj.org/toc/2041-1723Knowing the photophysics of thermally-activated delayed fluorescence (TADF) is crucial when designing organic light emitting diodes. Here the authors show that spin orbit coupling in TADF materials is described by a second order vibronic coupling mechanism, and demonstrate the importance of resonance effects to achieve efficient TADF.Marc K. EtheringtonJamie GibsonHeather F. HigginbothamThomas J. PenfoldAndrew P. MonkmanNature PortfolioarticleScienceQENNature Communications, Vol 7, Iss 1, Pp 1-7 (2016)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Marc K. Etherington Jamie Gibson Heather F. Higginbotham Thomas J. Penfold Andrew P. Monkman Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence
description	Knowing the photophysics of thermally-activated delayed fluorescence (TADF) is crucial when designing organic light emitting diodes. Here the authors show that spin orbit coupling in TADF materials is described by a second order vibronic coupling mechanism, and demonstrate the importance of resonance effects to achieve efficient TADF.
format	article
author	Marc K. Etherington Jamie Gibson Heather F. Higginbotham Thomas J. Penfold Andrew P. Monkman
author_facet	Marc K. Etherington Jamie Gibson Heather F. Higginbotham Thomas J. Penfold Andrew P. Monkman
author_sort	Marc K. Etherington
title	Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence
title_short	Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence
title_full	Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence
title_fullStr	Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence
title_full_unstemmed	Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence
title_sort	revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence
publisher	Nature Portfolio
publishDate	2016
url	https://doaj.org/article/3abe5e68e1034e658db51689cca04181
work_keys_str_mv	AT marcketherington revealingthespinvibroniccouplingmechanismofthermallyactivateddelayedfluorescence AT jamiegibson revealingthespinvibroniccouplingmechanismofthermallyactivateddelayedfluorescence AT heatherfhigginbotham revealingthespinvibroniccouplingmechanismofthermallyactivateddelayedfluorescence AT thomasjpenfold revealingthespinvibroniccouplingmechanismofthermallyactivateddelayedfluorescence AT andrewpmonkman revealingthespinvibroniccouplingmechanismofthermallyactivateddelayedfluorescence
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Revealing the spin–vibronic coupling mechanism of thermally activated delayed fluorescence

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