Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes

Solid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-...

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Main Authors:	Kevin N. Wood, K. Xerxes Steirer, Simon E. Hafner, Chunmei Ban, Shriram Santhanagopalan, Se-Hee Lee, Glenn Teeter
Format:	article
Language:	EN
Published:	Nature Portfolio 2018
Subjects:	Science Q
Online Access:	https://doaj.org/article/3b0325b8fd93416e85ed8fb7adb46f14
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spelling	oai:doaj.org-article:3b0325b8fd93416e85ed8fb7adb46f142021-12-02T17:32:45ZOperando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes10.1038/s41467-018-04762-z2041-1723https://doaj.org/article/3b0325b8fd93416e85ed8fb7adb46f142018-06-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-04762-zhttps://doaj.org/toc/2041-1723Solid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-electrolyte interphase during cycling.Kevin N. WoodK. Xerxes SteirerSimon E. HafnerChunmei BanShriram SanthanagopalanSe-Hee LeeGlenn TeeterNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-10 (2018)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Kevin N. Wood K. Xerxes Steirer Simon E. Hafner Chunmei Ban Shriram Santhanagopalan Se-Hee Lee Glenn Teeter Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
description	Solid-state electrolytes may improve the performance of batteries; however, many are unstable towards metallic lithium, and little is known about the chemical evolution of the interfaces that form during cycling. Here, the authors use an operando method to map the formation and evolution of a solid-electrolyte interphase during cycling.
format	article
author	Kevin N. Wood K. Xerxes Steirer Simon E. Hafner Chunmei Ban Shriram Santhanagopalan Se-Hee Lee Glenn Teeter
author_facet	Kevin N. Wood K. Xerxes Steirer Simon E. Hafner Chunmei Ban Shriram Santhanagopalan Se-Hee Lee Glenn Teeter
author_sort	Kevin N. Wood
title	Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_short	Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_full	Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_fullStr	Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_full_unstemmed	Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes
title_sort	operando x-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in li2s-p2s5 solid-state electrolytes
publisher	Nature Portfolio
publishDate	2018
url	https://doaj.org/article/3b0325b8fd93416e85ed8fb7adb46f14
work_keys_str_mv	AT kevinnwood operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT kxerxessteirer operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT simonehafner operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT chunmeiban operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT shriramsanthanagopalan operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT seheelee operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes AT glennteeter operandoxrayphotoelectronspectroscopyofsolidelectrolyteinterphaseformationandevolutioninli2sp2s5solidstateelectrolytes
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Operando X-ray photoelectron spectroscopy of solid electrolyte interphase formation and evolution in Li2S-P2S5 solid-state electrolytes

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