Selectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis

The reaction mechanism of carbon dioxide to high-value hydrocarbons over metal-zeolite bifunctional catalysts remains ambiguous. Here, the authors demonstrate that active zeolite catalysts’ topology and hybrid nature are descriptors; regulating the reaction mechanism and ultimate product selectivity...

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Autores principales: Adrian Ramirez, Xuan Gong, Mustafa Caglayan, Stefan-Adrian F. Nastase, Edy Abou-Hamad, Lieven Gevers, Luigi Cavallo, Abhishek Dutta Chowdhury, Jorge Gascon
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Publicado: Nature Portfolio 2021
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Acceso en línea:https://doaj.org/article/3d5c0f86e073499f885508bf2d550f02
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spelling oai:doaj.org-article:3d5c0f86e073499f885508bf2d550f022021-12-02T19:16:33ZSelectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis10.1038/s41467-021-26090-52041-1723https://doaj.org/article/3d5c0f86e073499f885508bf2d550f022021-10-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-26090-5https://doaj.org/toc/2041-1723The reaction mechanism of carbon dioxide to high-value hydrocarbons over metal-zeolite bifunctional catalysts remains ambiguous. Here, the authors demonstrate that active zeolite catalysts’ topology and hybrid nature are descriptors; regulating the reaction mechanism and ultimate product selectivity.Adrian RamirezXuan GongMustafa CaglayanStefan-Adrian F. NastaseEdy Abou-HamadLieven GeversLuigi CavalloAbhishek Dutta ChowdhuryJorge GasconNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-13 (2021)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Adrian Ramirez
Xuan Gong
Mustafa Caglayan
Stefan-Adrian F. Nastase
Edy Abou-Hamad
Lieven Gevers
Luigi Cavallo
Abhishek Dutta Chowdhury
Jorge Gascon
Selectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis
description The reaction mechanism of carbon dioxide to high-value hydrocarbons over metal-zeolite bifunctional catalysts remains ambiguous. Here, the authors demonstrate that active zeolite catalysts’ topology and hybrid nature are descriptors; regulating the reaction mechanism and ultimate product selectivity.
format article
author Adrian Ramirez
Xuan Gong
Mustafa Caglayan
Stefan-Adrian F. Nastase
Edy Abou-Hamad
Lieven Gevers
Luigi Cavallo
Abhishek Dutta Chowdhury
Jorge Gascon
author_facet Adrian Ramirez
Xuan Gong
Mustafa Caglayan
Stefan-Adrian F. Nastase
Edy Abou-Hamad
Lieven Gevers
Luigi Cavallo
Abhishek Dutta Chowdhury
Jorge Gascon
author_sort Adrian Ramirez
title Selectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis
title_short Selectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis
title_full Selectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis
title_fullStr Selectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis
title_full_unstemmed Selectivity descriptors for the direct hydrogenation of CO2 to hydrocarbons during zeolite-mediated bifunctional catalysis
title_sort selectivity descriptors for the direct hydrogenation of co2 to hydrocarbons during zeolite-mediated bifunctional catalysis
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/3d5c0f86e073499f885508bf2d550f02
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