Influence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System
Abstract We investigate the quantum optical properties of strong light-matter interaction between a quantum emitter and a metallic nanoparticle beyond idealized structures with a smooth surface. Based on the local coupling strength and macroscopic Green’s function, we derived an exact quantum optics...
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Nature Portfolio
2018
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oai:doaj.org-article:3e5f56bbeb04443bb7dbb9ef0354ea7e2021-12-02T11:40:24ZInfluence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System10.1038/s41598-018-25584-52045-2322https://doaj.org/article/3e5f56bbeb04443bb7dbb9ef0354ea7e2018-05-01T00:00:00Zhttps://doi.org/10.1038/s41598-018-25584-5https://doaj.org/toc/2045-2322Abstract We investigate the quantum optical properties of strong light-matter interaction between a quantum emitter and a metallic nanoparticle beyond idealized structures with a smooth surface. Based on the local coupling strength and macroscopic Green’s function, we derived an exact quantum optics approach to obtain the field enhancement and light-emission spectrum of a quantum emitter. Numerical simulations show that the surface roughness has a greater effect on the near-field than on the far-field, and slightly increases the vacuum Rabi splitting on average. Further, we verified that the near-field enhancement is mainly determined by the surface features of hot-spot area.Yu-Wei LuLing-Yan LiJing-Feng LiuNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 8, Iss 1, Pp 1-11 (2018) |
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Medicine R Science Q Yu-Wei Lu Ling-Yan Li Jing-Feng Liu Influence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System |
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Abstract We investigate the quantum optical properties of strong light-matter interaction between a quantum emitter and a metallic nanoparticle beyond idealized structures with a smooth surface. Based on the local coupling strength and macroscopic Green’s function, we derived an exact quantum optics approach to obtain the field enhancement and light-emission spectrum of a quantum emitter. Numerical simulations show that the surface roughness has a greater effect on the near-field than on the far-field, and slightly increases the vacuum Rabi splitting on average. Further, we verified that the near-field enhancement is mainly determined by the surface features of hot-spot area. |
format |
article |
author |
Yu-Wei Lu Ling-Yan Li Jing-Feng Liu |
author_facet |
Yu-Wei Lu Ling-Yan Li Jing-Feng Liu |
author_sort |
Yu-Wei Lu |
title |
Influence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System |
title_short |
Influence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System |
title_full |
Influence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System |
title_fullStr |
Influence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System |
title_full_unstemmed |
Influence of Surface Roughness on Strong Light-Matter Interaction of a Quantum Emitter-Metallic Nanoparticle System |
title_sort |
influence of surface roughness on strong light-matter interaction of a quantum emitter-metallic nanoparticle system |
publisher |
Nature Portfolio |
publishDate |
2018 |
url |
https://doaj.org/article/3e5f56bbeb04443bb7dbb9ef0354ea7e |
work_keys_str_mv |
AT yuweilu influenceofsurfaceroughnessonstronglightmatterinteractionofaquantumemittermetallicnanoparticlesystem AT lingyanli influenceofsurfaceroughnessonstronglightmatterinteractionofaquantumemittermetallicnanoparticlesystem AT jingfengliu influenceofsurfaceroughnessonstronglightmatterinteractionofaquantumemittermetallicnanoparticlesystem |
_version_ |
1718395636996374528 |