Fast room temperature lability of aluminosilicate zeolites

While aluminosilicate zeolites are of interest for many applications, the affect of water on zeolite stability in mild aqueous conditions has yet to be established. Here, using ab initio calculations and NMR spectroscopy, the authors show that covalent bonds in the zeolite chabazite are labile when...

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Auteurs principaux:	Christopher J. Heard, Lukas Grajciar, Cameron M. Rice, Suzi M. Pugh, Petr Nachtigall, Sharon E. Ashbrook, Russell E. Morris
Format:	article
Langue:	EN
Publié:	Nature Portfolio 2019
Sujets:	Science Q
Accès en ligne:	https://doaj.org/article/3fbdfc384c7b4d0b98913b793089d74f
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spelling	oai:doaj.org-article:3fbdfc384c7b4d0b98913b793089d74f2021-12-02T15:35:18ZFast room temperature lability of aluminosilicate zeolites10.1038/s41467-019-12752-y2041-1723https://doaj.org/article/3fbdfc384c7b4d0b98913b793089d74f2019-10-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-12752-yhttps://doaj.org/toc/2041-1723While aluminosilicate zeolites are of interest for many applications, the affect of water on zeolite stability in mild aqueous conditions has yet to be established. Here, using ab initio calculations and NMR spectroscopy, the authors show that covalent bonds in the zeolite chabazite are labile when in contact with neutral liquid water.Christopher J. HeardLukas GrajciarCameron M. RiceSuzi M. PughPetr NachtigallSharon E. AshbrookRussell E. MorrisNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-7 (2019)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Christopher J. Heard Lukas Grajciar Cameron M. Rice Suzi M. Pugh Petr Nachtigall Sharon E. Ashbrook Russell E. Morris Fast room temperature lability of aluminosilicate zeolites
description	While aluminosilicate zeolites are of interest for many applications, the affect of water on zeolite stability in mild aqueous conditions has yet to be established. Here, using ab initio calculations and NMR spectroscopy, the authors show that covalent bonds in the zeolite chabazite are labile when in contact with neutral liquid water.
format	article
author	Christopher J. Heard Lukas Grajciar Cameron M. Rice Suzi M. Pugh Petr Nachtigall Sharon E. Ashbrook Russell E. Morris
author_facet	Christopher J. Heard Lukas Grajciar Cameron M. Rice Suzi M. Pugh Petr Nachtigall Sharon E. Ashbrook Russell E. Morris
author_sort	Christopher J. Heard
title	Fast room temperature lability of aluminosilicate zeolites
title_short	Fast room temperature lability of aluminosilicate zeolites
title_full	Fast room temperature lability of aluminosilicate zeolites
title_fullStr	Fast room temperature lability of aluminosilicate zeolites
title_full_unstemmed	Fast room temperature lability of aluminosilicate zeolites
title_sort	fast room temperature lability of aluminosilicate zeolites
publisher	Nature Portfolio
publishDate	2019
url	https://doaj.org/article/3fbdfc384c7b4d0b98913b793089d74f
work_keys_str_mv	AT christopherjheard fastroomtemperaturelabilityofaluminosilicatezeolites AT lukasgrajciar fastroomtemperaturelabilityofaluminosilicatezeolites AT cameronmrice fastroomtemperaturelabilityofaluminosilicatezeolites AT suzimpugh fastroomtemperaturelabilityofaluminosilicatezeolites AT petrnachtigall fastroomtemperaturelabilityofaluminosilicatezeolites AT sharoneashbrook fastroomtemperaturelabilityofaluminosilicatezeolites AT russellemorris fastroomtemperaturelabilityofaluminosilicatezeolites
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Fast room temperature lability of aluminosilicate zeolites

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