Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
Catalytic transformation of CH4 under mild conditions has implications to shale gas utilization. Here, the authors report the transformation of CH4 to acetic acid through coupling of CH4, CO and O2 on single-site Rh1O5 anchored in microporous aluminosilicates in liquid phase.
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2018
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oai:doaj.org-article:43b30d1b051f4ed8b6ec301f45cab1492021-12-02T16:56:38ZSingle rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions10.1038/s41467-018-03235-72041-1723https://doaj.org/article/43b30d1b051f4ed8b6ec301f45cab1492018-03-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-03235-7https://doaj.org/toc/2041-1723Catalytic transformation of CH4 under mild conditions has implications to shale gas utilization. Here, the authors report the transformation of CH4 to acetic acid through coupling of CH4, CO and O2 on single-site Rh1O5 anchored in microporous aluminosilicates in liquid phase.Yu TangYuting LiVictor FungDe-en JiangWeixin HuangShiran ZhangYasuhiro IwasawaTomohiro SakataLuan NguyenXiaoyan ZhangAnatoly I. FrenkelFranklin (Feng) TaoNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-11 (2018) |
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Science Q Yu Tang Yuting Li Victor Fung De-en Jiang Weixin Huang Shiran Zhang Yasuhiro Iwasawa Tomohiro Sakata Luan Nguyen Xiaoyan Zhang Anatoly I. Frenkel Franklin (Feng) Tao Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions |
description |
Catalytic transformation of CH4 under mild conditions has implications to shale gas utilization. Here, the authors report the transformation of CH4 to acetic acid through coupling of CH4, CO and O2 on single-site Rh1O5 anchored in microporous aluminosilicates in liquid phase. |
format |
article |
author |
Yu Tang Yuting Li Victor Fung De-en Jiang Weixin Huang Shiran Zhang Yasuhiro Iwasawa Tomohiro Sakata Luan Nguyen Xiaoyan Zhang Anatoly I. Frenkel Franklin (Feng) Tao |
author_facet |
Yu Tang Yuting Li Victor Fung De-en Jiang Weixin Huang Shiran Zhang Yasuhiro Iwasawa Tomohiro Sakata Luan Nguyen Xiaoyan Zhang Anatoly I. Frenkel Franklin (Feng) Tao |
author_sort |
Yu Tang |
title |
Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions |
title_short |
Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions |
title_full |
Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions |
title_fullStr |
Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions |
title_full_unstemmed |
Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions |
title_sort |
single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions |
publisher |
Nature Portfolio |
publishDate |
2018 |
url |
https://doaj.org/article/43b30d1b051f4ed8b6ec301f45cab149 |
work_keys_str_mv |
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