Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions

Catalytic transformation of CH4 under mild conditions has implications to shale gas utilization. Here, the authors report the transformation of CH4 to acetic acid through coupling of CH4, CO and O2 on single-site Rh1O5 anchored in microporous aluminosilicates in liquid phase.

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Autores principales:	Yu Tang, Yuting Li, Victor Fung, De-en Jiang, Weixin Huang, Shiran Zhang, Yasuhiro Iwasawa, Tomohiro Sakata, Luan Nguyen, Xiaoyan Zhang, Anatoly I. Frenkel, Franklin (Feng) Tao
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2018
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/43b30d1b051f4ed8b6ec301f45cab149
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spelling	oai:doaj.org-article:43b30d1b051f4ed8b6ec301f45cab1492021-12-02T16:56:38ZSingle rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions10.1038/s41467-018-03235-72041-1723https://doaj.org/article/43b30d1b051f4ed8b6ec301f45cab1492018-03-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-03235-7https://doaj.org/toc/2041-1723Catalytic transformation of CH4 under mild conditions has implications to shale gas utilization. Here, the authors report the transformation of CH4 to acetic acid through coupling of CH4, CO and O2 on single-site Rh1O5 anchored in microporous aluminosilicates in liquid phase.Yu TangYuting LiVictor FungDe-en JiangWeixin HuangShiran ZhangYasuhiro IwasawaTomohiro SakataLuan NguyenXiaoyan ZhangAnatoly I. FrenkelFranklin (Feng) TaoNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-11 (2018)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Yu Tang Yuting Li Victor Fung De-en Jiang Weixin Huang Shiran Zhang Yasuhiro Iwasawa Tomohiro Sakata Luan Nguyen Xiaoyan Zhang Anatoly I. Frenkel Franklin (Feng) Tao Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
description	Catalytic transformation of CH4 under mild conditions has implications to shale gas utilization. Here, the authors report the transformation of CH4 to acetic acid through coupling of CH4, CO and O2 on single-site Rh1O5 anchored in microporous aluminosilicates in liquid phase.
format	article
author	Yu Tang Yuting Li Victor Fung De-en Jiang Weixin Huang Shiran Zhang Yasuhiro Iwasawa Tomohiro Sakata Luan Nguyen Xiaoyan Zhang Anatoly I. Frenkel Franklin (Feng) Tao
author_facet	Yu Tang Yuting Li Victor Fung De-en Jiang Weixin Huang Shiran Zhang Yasuhiro Iwasawa Tomohiro Sakata Luan Nguyen Xiaoyan Zhang Anatoly I. Frenkel Franklin (Feng) Tao
author_sort	Yu Tang
title	Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
title_short	Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
title_full	Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
title_fullStr	Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
title_full_unstemmed	Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
title_sort	single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
publisher	Nature Portfolio
publishDate	2018
url	https://doaj.org/article/43b30d1b051f4ed8b6ec301f45cab149
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Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions

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