High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy

Abstract High-sensitivity detection of hydrogen (H) contained in zircaloy-4, a commonly used material for nuclear fuel containers, is crucial in a nuclear power plant. Currently, H detection is performed via gas chromatography, which is an offline and destructive method. In this study, we developed...

Descripción completa

Guardado en:

Detalles Bibliográficos
Autores principales:	Marincan Pardede, Indra Karnadi, Rinda Hedwig, Ivan Tanra, Javed Iqbal, Mangasi Alion Marpaung, Maria Margaretha Suliyanti, Eric Jobiliong, Syahrun Nur Abdulmadjid, Nasrullah Idris, Ali Khumaeni, Muhandis Shiddiq, Mario Gracio Anduinta Rhizma, Zener Sukra Lie, Muhammad Bilal, Davy Putra Kurniawan, Tjung Jie Lie, Koo Hendrik Kurniawan, Kiichiro Kagawa
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2021
Materias:	Medicine R Science Q
Acceso en línea:	https://doaj.org/article/4439f8c74afa40989646c96e47dae667
Etiquetas:	Agregar Etiqueta Sin Etiquetas, Sea el primero en etiquetar este registro!

id	oai:doaj.org-article:4439f8c74afa40989646c96e47dae667
record_format	dspace
spelling	oai:doaj.org-article:4439f8c74afa40989646c96e47dae6672021-11-14T12:22:14ZHigh sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy10.1038/s41598-021-01601-y2045-2322https://doaj.org/article/4439f8c74afa40989646c96e47dae6672021-11-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-01601-yhttps://doaj.org/toc/2045-2322Abstract High-sensitivity detection of hydrogen (H) contained in zircaloy-4, a commonly used material for nuclear fuel containers, is crucial in a nuclear power plant. Currently, H detection is performed via gas chromatography, which is an offline and destructive method. In this study, we developed a technique based on metastable excited-state He-assisted excitation to achieve excellent quality of H emission spectra in double-pulse orthogonal laser-induced breakdown spectroscopy (LIBS). The production of metastable excited-state He atoms is optimized by using LiF as sub-target material. The results show a narrow full-width-at-half-maximum of 0.5 Å for the H I 656.2 nm emission line, with a detection limit as low as 0.51 mg/kg. Thus, using this novel online method, H in zircaloy-4 can be detected efficiently, even at very low concentrations.Marincan PardedeIndra KarnadiRinda HedwigIvan TanraJaved IqbalMangasi Alion MarpaungMaria Margaretha SuliyantiEric JobiliongSyahrun Nur AbdulmadjidNasrullah IdrisAli KhumaeniMuhandis ShiddiqMario Gracio Anduinta RhizmaZener Sukra LieMuhammad BilalDavy Putra KurniawanTjung Jie LieKoo Hendrik KurniawanKiichiro KagawaNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-10 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	Medicine R Science Q
spellingShingle	Medicine R Science Q Marincan Pardede Indra Karnadi Rinda Hedwig Ivan Tanra Javed Iqbal Mangasi Alion Marpaung Maria Margaretha Suliyanti Eric Jobiliong Syahrun Nur Abdulmadjid Nasrullah Idris Ali Khumaeni Muhandis Shiddiq Mario Gracio Anduinta Rhizma Zener Sukra Lie Muhammad Bilal Davy Putra Kurniawan Tjung Jie Lie Koo Hendrik Kurniawan Kiichiro Kagawa High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy
description	Abstract High-sensitivity detection of hydrogen (H) contained in zircaloy-4, a commonly used material for nuclear fuel containers, is crucial in a nuclear power plant. Currently, H detection is performed via gas chromatography, which is an offline and destructive method. In this study, we developed a technique based on metastable excited-state He-assisted excitation to achieve excellent quality of H emission spectra in double-pulse orthogonal laser-induced breakdown spectroscopy (LIBS). The production of metastable excited-state He atoms is optimized by using LiF as sub-target material. The results show a narrow full-width-at-half-maximum of 0.5 Å for the H I 656.2 nm emission line, with a detection limit as low as 0.51 mg/kg. Thus, using this novel online method, H in zircaloy-4 can be detected efficiently, even at very low concentrations.
format	article
author	Marincan Pardede Indra Karnadi Rinda Hedwig Ivan Tanra Javed Iqbal Mangasi Alion Marpaung Maria Margaretha Suliyanti Eric Jobiliong Syahrun Nur Abdulmadjid Nasrullah Idris Ali Khumaeni Muhandis Shiddiq Mario Gracio Anduinta Rhizma Zener Sukra Lie Muhammad Bilal Davy Putra Kurniawan Tjung Jie Lie Koo Hendrik Kurniawan Kiichiro Kagawa
author_facet	Marincan Pardede Indra Karnadi Rinda Hedwig Ivan Tanra Javed Iqbal Mangasi Alion Marpaung Maria Margaretha Suliyanti Eric Jobiliong Syahrun Nur Abdulmadjid Nasrullah Idris Ali Khumaeni Muhandis Shiddiq Mario Gracio Anduinta Rhizma Zener Sukra Lie Muhammad Bilal Davy Putra Kurniawan Tjung Jie Lie Koo Hendrik Kurniawan Kiichiro Kagawa
author_sort	Marincan Pardede
title	High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy
title_short	High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy
title_full	High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy
title_fullStr	High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy
title_full_unstemmed	High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy
title_sort	high sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy
publisher	Nature Portfolio
publishDate	2021
url	https://doaj.org/article/4439f8c74afa40989646c96e47dae667
work_keys_str_mv	AT marincanpardede highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT indrakarnadi highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT rindahedwig highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT ivantanra highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT javediqbal highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT mangasialionmarpaung highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT mariamargarethasuliyanti highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT ericjobiliong highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT syahrunnurabdulmadjid highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT nasrullahidris highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT alikhumaeni highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT muhandisshiddiq highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT mariogracioanduintarhizma highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT zenersukralie highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT muhammadbilal highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT davyputrakurniawan highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT tjungjielie highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT koohendrikkurniawan highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy AT kiichirokagawa highsensitivityhydrogenanalysisinzircaloy4usingheliumassistedexcitationlaserinducedbreakdownspectroscopy
_version_	1718429222057279488

High sensitivity hydrogen analysis in zircaloy-4 using helium-assisted excitation laser-induced breakdown spectroscopy

Ejemplares similares