Vibronic coherence evolution in multidimensional ultrafast photochemical processes
Energy transfer in light harvesting complexes involves electronic, vibrational, and vibronic couplings which are challenging to resolve. Here the authors observe the time-evolution of vibronic coherences driving charge transfer in a photoexcited solvated transition metal complex by two- and three-di...
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Nature Portfolio
2019
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oai:doaj.org-article:44f0bc61b83e4eeb9d596961142a6fc62021-12-02T13:23:54ZVibronic coherence evolution in multidimensional ultrafast photochemical processes10.1038/s41467-019-13503-92041-1723https://doaj.org/article/44f0bc61b83e4eeb9d596961142a6fc62019-12-01T00:00:00Zhttps://doi.org/10.1038/s41467-019-13503-9https://doaj.org/toc/2041-1723Energy transfer in light harvesting complexes involves electronic, vibrational, and vibronic couplings which are challenging to resolve. Here the authors observe the time-evolution of vibronic coherences driving charge transfer in a photoexcited solvated transition metal complex by two- and three-dimensional electronic-vibrational spectroscopy.James D. GaynorJason SandwischMunira KhalilNature PortfolioarticleScienceQENNature Communications, Vol 10, Iss 1, Pp 1-9 (2019) |
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Science Q James D. Gaynor Jason Sandwisch Munira Khalil Vibronic coherence evolution in multidimensional ultrafast photochemical processes |
description |
Energy transfer in light harvesting complexes involves electronic, vibrational, and vibronic couplings which are challenging to resolve. Here the authors observe the time-evolution of vibronic coherences driving charge transfer in a photoexcited solvated transition metal complex by two- and three-dimensional electronic-vibrational spectroscopy. |
format |
article |
author |
James D. Gaynor Jason Sandwisch Munira Khalil |
author_facet |
James D. Gaynor Jason Sandwisch Munira Khalil |
author_sort |
James D. Gaynor |
title |
Vibronic coherence evolution in multidimensional ultrafast photochemical processes |
title_short |
Vibronic coherence evolution in multidimensional ultrafast photochemical processes |
title_full |
Vibronic coherence evolution in multidimensional ultrafast photochemical processes |
title_fullStr |
Vibronic coherence evolution in multidimensional ultrafast photochemical processes |
title_full_unstemmed |
Vibronic coherence evolution in multidimensional ultrafast photochemical processes |
title_sort |
vibronic coherence evolution in multidimensional ultrafast photochemical processes |
publisher |
Nature Portfolio |
publishDate |
2019 |
url |
https://doaj.org/article/44f0bc61b83e4eeb9d596961142a6fc6 |
work_keys_str_mv |
AT jamesdgaynor vibroniccoherenceevolutioninmultidimensionalultrafastphotochemicalprocesses AT jasonsandwisch vibroniccoherenceevolutioninmultidimensionalultrafastphotochemicalprocesses AT munirakhalil vibroniccoherenceevolutioninmultidimensionalultrafastphotochemicalprocesses |
_version_ |
1718393145958334464 |