Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water

Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with...

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Autores principales: Yiou Wang, Xu Liu, Xiaoyu Han, Robert Godin, Jialu Chen, Wuzong Zhou, Chaoran Jiang, Jamie F. Thompson, K. Bayazit Mustafa, Stephen A. Shevlin, James R. Durrant, Zhengxiao Guo, Junwang Tang
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Lenguaje:EN
Publicado: Nature Portfolio 2020
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Acceso en línea:https://doaj.org/article/455d9001207c44ddbeb635584c223a1c
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spelling oai:doaj.org-article:455d9001207c44ddbeb635584c223a1c2021-12-02T14:58:44ZUnique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water10.1038/s41467-020-16227-32041-1723https://doaj.org/article/455d9001207c44ddbeb635584c223a1c2020-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-16227-3https://doaj.org/toc/2041-1723Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with nearly 100% selectivity to methanol.Yiou WangXu LiuXiaoyu HanRobert GodinJialu ChenWuzong ZhouChaoran JiangJamie F. ThompsonK. Bayazit MustafaStephen A. ShevlinJames R. DurrantZhengxiao GuoJunwang TangNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-9 (2020)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Yiou Wang
Xu Liu
Xiaoyu Han
Robert Godin
Jialu Chen
Wuzong Zhou
Chaoran Jiang
Jamie F. Thompson
K. Bayazit Mustafa
Stephen A. Shevlin
James R. Durrant
Zhengxiao Guo
Junwang Tang
Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
description Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with nearly 100% selectivity to methanol.
format article
author Yiou Wang
Xu Liu
Xiaoyu Han
Robert Godin
Jialu Chen
Wuzong Zhou
Chaoran Jiang
Jamie F. Thompson
K. Bayazit Mustafa
Stephen A. Shevlin
James R. Durrant
Zhengxiao Guo
Junwang Tang
author_facet Yiou Wang
Xu Liu
Xiaoyu Han
Robert Godin
Jialu Chen
Wuzong Zhou
Chaoran Jiang
Jamie F. Thompson
K. Bayazit Mustafa
Stephen A. Shevlin
James R. Durrant
Zhengxiao Guo
Junwang Tang
author_sort Yiou Wang
title Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
title_short Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
title_full Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
title_fullStr Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
title_full_unstemmed Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
title_sort unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
publisher Nature Portfolio
publishDate 2020
url https://doaj.org/article/455d9001207c44ddbeb635584c223a1c
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