Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water
Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with...
Guardado en:
Autores principales: | , , , , , , , , , , , , |
---|---|
Formato: | article |
Lenguaje: | EN |
Publicado: |
Nature Portfolio
2020
|
Materias: | |
Acceso en línea: | https://doaj.org/article/455d9001207c44ddbeb635584c223a1c |
Etiquetas: |
Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
|
id |
oai:doaj.org-article:455d9001207c44ddbeb635584c223a1c |
---|---|
record_format |
dspace |
spelling |
oai:doaj.org-article:455d9001207c44ddbeb635584c223a1c2021-12-02T14:58:44ZUnique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water10.1038/s41467-020-16227-32041-1723https://doaj.org/article/455d9001207c44ddbeb635584c223a1c2020-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-16227-3https://doaj.org/toc/2041-1723Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with nearly 100% selectivity to methanol.Yiou WangXu LiuXiaoyu HanRobert GodinJialu ChenWuzong ZhouChaoran JiangJamie F. ThompsonK. Bayazit MustafaStephen A. ShevlinJames R. DurrantZhengxiao GuoJunwang TangNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-9 (2020) |
institution |
DOAJ |
collection |
DOAJ |
language |
EN |
topic |
Science Q |
spellingShingle |
Science Q Yiou Wang Xu Liu Xiaoyu Han Robert Godin Jialu Chen Wuzong Zhou Chaoran Jiang Jamie F. Thompson K. Bayazit Mustafa Stephen A. Shevlin James R. Durrant Zhengxiao Guo Junwang Tang Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water |
description |
Solar-driven CO2 reduction by abundant water to alcohols is hindered by the sluggish water oxidation reaction. Here, the authors demonstrate that the microwave-synthesized carbon-dots possess unique hole-accepting nature, allowing stoichiometric oxygen and methanol production from water and CO2 with nearly 100% selectivity to methanol. |
format |
article |
author |
Yiou Wang Xu Liu Xiaoyu Han Robert Godin Jialu Chen Wuzong Zhou Chaoran Jiang Jamie F. Thompson K. Bayazit Mustafa Stephen A. Shevlin James R. Durrant Zhengxiao Guo Junwang Tang |
author_facet |
Yiou Wang Xu Liu Xiaoyu Han Robert Godin Jialu Chen Wuzong Zhou Chaoran Jiang Jamie F. Thompson K. Bayazit Mustafa Stephen A. Shevlin James R. Durrant Zhengxiao Guo Junwang Tang |
author_sort |
Yiou Wang |
title |
Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water |
title_short |
Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water |
title_full |
Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water |
title_fullStr |
Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water |
title_full_unstemmed |
Unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water |
title_sort |
unique hole-accepting carbon-dots promoting selective carbon dioxide reduction nearly 100% to methanol by pure water |
publisher |
Nature Portfolio |
publishDate |
2020 |
url |
https://doaj.org/article/455d9001207c44ddbeb635584c223a1c |
work_keys_str_mv |
AT yiouwang uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT xuliu uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT xiaoyuhan uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT robertgodin uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT jialuchen uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT wuzongzhou uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT chaoranjiang uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT jamiefthompson uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT kbayazitmustafa uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT stephenashevlin uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT jamesrdurrant uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT zhengxiaoguo uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater AT junwangtang uniqueholeacceptingcarbondotspromotingselectivecarbondioxidereductionnearly100tomethanolbypurewater |
_version_ |
1718389262022344704 |